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We herein identify a straightforward synthetic strategy towards universal hydrogen\u2010bonded (H\u2010bonded) polymeric adhesives, using a side\u2010chain barbiturate (Ba) and Hamilton wedge (HW) functionalized copolymer. Starting from a rubbery copolymer containing thiolactone derivatives, Ba and HW moieties are tethered as pendant groups via an efficient one\u2010pot two\u2010step amine\u2010thiol\u2010bromo conjugation. Hetero\u2010complementary Ba\/HW interactions thus yield H\u2010bonded supramolecular polymeric networks. In addition to an enhanced polymeric network integrity induced by specific Ba\/HW association, the presence of individual Ba or HW moieties enables strong binding to a range of substrates, outstanding compared to commercial glues and reported adhesives.<\/jats:p>","DOI":"10.1002\/anie.202203876","type":"journal-article","created":{"date-parts":[[2022,4,15]],"date-time":"2022-04-15T04:19:40Z","timestamp":1649996380000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":85,"title":["Hydrogen\u2010Bonded Supramolecular Polymer Adhesives: Straightforward Synthesis and Strong Substrate Interaction"],"prefix":"10.1002","volume":"61","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-5599-6819","authenticated-orcid":false,"given":"Senbin","family":"Chen","sequence":"first","affiliation":[{"name":"Key Laboratory of Materials Chemistry for Energy Conversion and Storage Ministry of Education (HUST) School of Chemistry and Chemical Engineering Huazhong University of Science and Technology (HUST)  Wuhan 430074 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zeke","family":"Li","sequence":"additional","affiliation":[{"name":"Key Laboratory of Materials Chemistry for Energy Conversion and Storage Ministry of Education (HUST) School of Chemistry and Chemical Engineering Huazhong University of Science and Technology (HUST)  Wuhan 430074 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanggui","family":"Wu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Materials Chemistry for Energy Conversion and Storage Ministry of Education (HUST) School of Chemistry and Chemical Engineering Huazhong University of Science and Technology (HUST)  Wuhan 430074 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nasir","family":"Mahmood","sequence":"additional","affiliation":[{"name":"Institute of Chemistry, Chair of Macromolecular Chemistry Faculty of Natural Sciences II Martin-Luther University Halle-Wittenberg  Kurth-Mothes-Strasse 2 06120 Halle (Saale) Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fr\u00e9d\u00e9ric","family":"Lortie","sequence":"additional","affiliation":[{"name":"Universit\u00e9 de Lyon, CNRS, UMR 5223, Ing\u00e9nierie des Mat\u00e9riaux Polym\u00e8res  Universit\u00e9 Lyon 1, INSA Lyon, UJM 69621 Villeurbanne cedex France"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Julien","family":"Bernard","sequence":"additional","affiliation":[{"name":"Universit\u00e9 de Lyon, CNRS, UMR 5223, Ing\u00e9nierie des Mat\u00e9riaux Polym\u00e8res  Universit\u00e9 Lyon 1, INSA Lyon, UJM 69621 Villeurbanne cedex France"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wolfgang H.","family":"Binder","sequence":"additional","affiliation":[{"name":"Institute of Chemistry Martin-Luther University Halle-Wittenberg  von Danckelmann-Platz 4 06120 Halle Saale) Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jintao","family":"Zhu","sequence":"additional","affiliation":[{"name":"Key Laboratory of Materials Chemistry for Energy Conversion and Storage Ministry of Education (HUST) School of Chemistry and Chemical Engineering Huazhong University of Science and Technology (HUST)  Wuhan 430074 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2022,5,3]]},"reference":[{"key":"e_1_2_7_1_1","doi-asserted-by":"publisher","DOI":"10.1038\/35015073"},{"key":"e_1_2_7_2_1","doi-asserted-by":"publisher","DOI":"10.1098\/rsfs.2014.0086"},{"key":"e_1_2_7_3_1","doi-asserted-by":"publisher","DOI":"10.1039\/C8CS00955D"},{"key":"e_1_2_7_4_1","first-page":"e1012","volume":"1","author":"Shi C.-Y.","year":"2020","journal-title":"Smart Mater. 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