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However, the interactions between solvent\/solvent molecules and solvent\/polymer chains are usually ignored. Herein, a series of ultra\u2010tough ionogels were prepared via a supramolecular solvent, halometallate ionic liquid, in which cations and coordinating anions form a 3D supramolecular network. The linear polymer chains are physically cross\u2010linked with supramolecular solvents synergistically enhancing the strength (14.3\u2005MPa), toughness (78\u2005MJ\u2009m\n                    <jats:sup>\u22123<\/jats:sup>\n                    ), and Young's modulus (55\u2005MPa) of ionogels, effectively dispersing the stress concentration under load, and obtaining better fatigue resistance and higher fracture energy (198\u2005kJ\u2009m\n                    <jats:sup>\u22122<\/jats:sup>\n                    ). Furthermore, the reversible cross\u2010linking enables green recovery and recycling of ionogels, simply by water. This strategy shows broad applicability based on a variety of supramolecular solvents and coordinatable polymers.\n                  <\/jats:p>","DOI":"10.1002\/anie.202212512","type":"journal-article","created":{"date-parts":[[2022,10,20]],"date-time":"2022-10-20T08:50:32Z","timestamp":1666255832000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":166,"title":["Ultra\u2010Tough and Recyclable Ionogels Constructed by Coordinated Supramolecular Solvents"],"prefix":"10.1002","volume":"61","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-1880-9356","authenticated-orcid":false,"given":"Lingling","family":"Li","sequence":"first","affiliation":[{"name":"Jiangsu Engineering Laboratory of Novel Functional Polymeric Materials Jiangsu Key Laboratory of Advanced Negative Carbon Technologies College of Chemistry Suzhou Key Laboratory of Soft Material and New Energy College of Chemistry Chemical Engineering and Materials Science Soochow 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