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The experimental studies are complemented by density functional theory calculations, proving that the pyrene unit is more active for H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    production than the bipyridine and (diarylamino)benzene units reported previously. H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    decomposition experiments verified that the distribution of pyrene units over a large surface area of COFs plays an important role in catalytic performance. The Py\u2010Py\u2010COF though contains more pyrene units than other COFs which induces a high H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    decomposition due to a dense concentration of pyrene in close proximity over a limited surface area. Therefore, a two\u2010phase reaction system (water\u2010benzyl alcohol) was employed to inhibit H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    decomposition. This is the first report on applying pyrene\u2010based COFs in a two\u2010phase system for photocatalytic H\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    generation.\n                  <\/jats:p>","DOI":"10.1002\/anie.202216719","type":"journal-article","created":{"date-parts":[[2023,3,10]],"date-time":"2023-03-10T11:05:25Z","timestamp":1678446325000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":284,"title":["Pyrene\u2010Based Covalent Organic Frameworks for Photocatalytic Hydrogen Peroxide Production"],"prefix":"10.1002","volume":"62","author":[{"given":"Jiamin","family":"Sun","sequence":"first","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Himanshu","family":"Sekhar Jena","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chidharth","family":"Krishnaraj","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kuber","family":"Singh Rawat","sequence":"additional","affiliation":[{"name":"Center for Molecular Modeling (CMM) Ghent University  Technologiepark 46 9052 Zwijnaarde Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sara","family":"Abednatanzi","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jeet","family":"Chakraborty","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Andreas","family":"Laemont","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wanlu","family":"Liu","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hui","family":"Chen","sequence":"additional","affiliation":[{"name":"COMOC\u2014Center for Ordered Materials Organometallics and Catalysis Department of Chemistry Ghent University  Krijgslaan 281, building S3 9000 Ghent Belgium"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ying\u2010Ya","family":"Liu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Fine Chemicals Dalian University of Technology  116023 Dalian P. 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