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Manipulating the nucleation mode and deposition orientation of Zn is a key to rendering stabilized Zn anodes. Here, a dual electrolyte additive strategy is put forward via the direct cooperation of xylitol (XY) and graphene oxide (GO) species into typical zinc sulfate electrolyte. As verified by molecular dynamics simulations, the incorporated XY molecules could regulate the solvation structure of Zn<jats:sup>2+<\/jats:sup>, thus inhibiting hydrogen evolution and side reactions. The self\u2010assembled GO layer is in favor of facilitating the desolvation process to accelerate reaction kinetics. Progressive nucleation and orientational deposition can be realized under the synergistic modulation, enabling a dense and uniform Zn deposition. Consequently, symmetric cell based on dual additives harvests a highly reversible cycling of 5600\u2005h at 1.0\u2005mA\u2009cm<jats:sup>\u22122<\/jats:sup>\/1.0\u2005mAh\u2009cm<jats:sup>\u22122<\/jats:sup>.<\/jats:p>","DOI":"10.1002\/anie.202218454","type":"journal-article","created":{"date-parts":[[2023,1,10]],"date-time":"2023-01-10T03:18:58Z","timestamp":1673320738000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":166,"title":["Synchronous Dual Electrolyte Additive Sustains Zn Metal Anode with 5600\u2005h Lifespan"],"prefix":"10.1002","volume":"62","author":[{"given":"Xianzhong","family":"Yang","sequence":"first","affiliation":[{"name":"College of Energy Soochow Institute for Energy and Materials Innovations Jiangsu Provincial Key Laboratory for Advanced Carbon Materials and Wearable Energy Technologies Soochow University Suzhou 215006 P. R. 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