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Herein, we first report the synthesis of nitrogen\u2010doped BiOCl atomic layers to directly split carbon\u2010sequestrated natural seawater (Yellow Sea, China) into stoichiometric CO (92.8\u2005\u03bcmol\u2009h\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) and HClO (83.2\u2005\u03bcmol\u2009h\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) under visible light with selectivities greater than 90\u2009%. Photoelectrons enriched on the exposed BiOCl{001} facet kinetically facilitate CO\n                    <jats:sub>2<\/jats:sub>\n                    \u2010to\u2010CO reduction\n                    <jats:italic>via<\/jats:italic>\n                    surface\u2010doped nitrogen bearing Lewis basicity. Photoholes, mainly located on the lateral facets of van der Waals gaps, promote the selective oxidation of Cl\n                    <jats:sup>\u2212<\/jats:sup>\n                    into HClO. Sequestrated CO\n                    <jats:sub>2<\/jats:sub>\n                    also maintains the pH of seawater at around 4.2 to prevent the alkaline earth cations from precipitating. The produced HClO can effectively kill typical bacteria in the ballast water of ocean\u2010going cargo ships, offering a green and safe way for onsite sterilization.\n                  <\/jats:p>","DOI":"10.1002\/anie.202302286","type":"journal-article","created":{"date-parts":[[2023,4,17]],"date-time":"2023-04-17T10:08:40Z","timestamp":1681726120000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":103,"title":["Visible Light\u2010Driven Conversion of Carbon\u2010Sequestrated Seawater into Stoichiometric CO and HClO with Nitrogen\u2010Doped BiOCl Atomic Layers"],"prefix":"10.1002","volume":"62","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3137-9837","authenticated-orcid":false,"given":"Yanbiao","family":"Shi","sequence":"first","affiliation":[{"name":"School of Environmental Science and Engineering Shanghai Jiao Tong University  Shanghai 200240 P. R. 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