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However, the narrow interlayer spacing, low intrinsic conductivity and the vanadium dissolution still restrict their further application. Herein, we present an oxygen\u2010deficient vanadate pillared by carbon nitride (C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    ) as the cathode for AZIBs through a facile self\u2010engaged hydrothermal strategy. Of note, C\n                    <jats:sub>3<\/jats:sub>\n                    N\n                    <jats:sub>4<\/jats:sub>\n                    nanosheets can act as both the nitrogen source and pre\u2010intercalation species to transform the orthorhombic V\n                    <jats:sub>2<\/jats:sub>\n                    O\n                    <jats:sub>5<\/jats:sub>\n                    into layered NH\n                    <jats:sub>4<\/jats:sub>\n                    V\n                    <jats:sub>4<\/jats:sub>\n                    O\n                    <jats:sub>10<\/jats:sub>\n                    with expanded interlayer spacing. Owing to the pillared structure and abundant oxygen vacancies, both the Zn\n                    <jats:sup>2+<\/jats:sup>\n                    ion (de)intercalation kinetics and the ionic conductivity in the NH\n                    <jats:sub>4<\/jats:sub>\n                    V\n                    <jats:sub>4<\/jats:sub>\n                    O\n                    <jats:sub>10<\/jats:sub>\n                    cathode are promoted. As a result, the NH\n                    <jats:sub>4<\/jats:sub>\n                    V\n                    <jats:sub>4<\/jats:sub>\n                    O\n                    <jats:sub>10<\/jats:sub>\n                    cathode delivers exceptional Zn\u2010ion storage ability with a high specific capacity of about 370\u2005mAh\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    at 0.5\u2005A\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , a high\u2010rate capability of 194.7\u2005mAh\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    at 20\u2005A\u2009g\n                    <jats:sup>\u22121<\/jats:sup>\n                    and a stable cycling performance of 10\u2009000\u2005cycles.\n                  <\/jats:p>","DOI":"10.1002\/anie.202303529","type":"journal-article","created":{"date-parts":[[2023,5,3]],"date-time":"2023-05-03T07:31:02Z","timestamp":1683099062000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":115,"title":["Carbon Nitride Pillared Vanadate Via Chemical Pre\u2010Intercalation Towards High\u2010Performance Aqueous Zinc\u2010Ion Batteries"],"prefix":"10.1002","volume":"62","author":[{"given":"Yue","family":"Xu","sequence":"first","affiliation":[{"name":"School of Chemistry and Chemical Engineering Inner Mongolia University  010021 Hohhot China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guilan","family":"Fan","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Inner Mongolia University  010021 Hohhot China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Peng Xiao","family":"Sun","sequence":"additional","affiliation":[{"name":"State Key Lab of Organic-Inorganic Composites Beijing University of Chemical Technology  100029 Beijing P.\u2005R. 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