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Here, we present the development of a polymer\u2010matrixed zeolite separator (SZ) by synthesizing zeolite materials on a flexible polymeric membrane. This separator acts as an effective ionic barrier, preventing the leaching and shuttling of vanadium from the cathode, while significantly inhibiting the formation of by\u2010products and zinc dendrites. The SZ cells demonstrate stable operation for more than 400\u2005cycles at 0.5\u2005A\u2009g<jats:sup>\u22121<\/jats:sup>, with an initial capacity of 375.4\u2005mAh\u2009g<jats:sup>\u22121<\/jats:sup>, and over 10,000\u2005cycles at 15\u2005A\u2009g<jats:sup>\u22121<\/jats:sup>. Notably, when pre\u2010anchored with vanadium ions, the SZ\u2010V cells exhibited excellent capacity retention of up to 94.6\u2009% over 1000\u2005cycles. The SZ separator featuring an ion barrier represents a crucial advancement towards the commercialization of zinc storage devices.<\/jats:p>","DOI":"10.1002\/anie.202315464","type":"journal-article","created":{"date-parts":[[2023,11,30]],"date-time":"2023-11-30T15:45:50Z","timestamp":1701359150000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":83,"title":["Preventing Dissolution of Cathode Active Materials by Ion\u2010anchoring Zeolite\u2010based Separators for Durable Aqueous Zinc Batteries**"],"prefix":"10.1002","volume":"63","author":[{"given":"Yao","family":"Qin","sequence":"first","affiliation":[{"name":"Songshan Lake Materials Laboratory  Dongguan, Guangdong 523808 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5366-9918","authenticated-orcid":false,"given":"Xin","family":"Wang","sequence":"additional","affiliation":[{"name":"Songshan Lake Materials Laboratory  Dongguan, Guangdong 523808 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2023,12,11]]},"reference":[{"key":"e_1_2_7_1_1","unstructured":"\u00a0"},{"key":"e_1_2_7_2_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2023.05.004"},{"key":"e_1_2_7_3_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41893-022-01028-x"},{"key":"e_1_2_7_4_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.2c06757"},{"key":"e_1_2_7_5_1","unstructured":"\u00a0"},{"key":"e_1_2_7_6_2","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202207118"},{"key":"e_1_2_7_7_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41565-021-00905-4"},{"key":"e_1_2_7_8_1","unstructured":"\u00a0"},{"key":"e_1_2_7_9_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41893-022-00919-3"},{"key":"e_1_2_7_10_2","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.202202039"},{"key":"e_1_2_7_11_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202304036"},{"key":"e_1_2_7_12_1","unstructured":"\u00a0"},{"key":"e_1_2_7_13_2","doi-asserted-by":"publisher","DOI":"10.1021\/acsnano.2c04968"},{"key":"e_1_2_7_14_2","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202213187"},{"key":"e_1_2_7_15_1","unstructured":"\u00a0"},{"key":"e_1_2_7_16_2","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202109671"},{"key":"e_1_2_7_17_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-29987-x"},{"key":"e_1_2_7_18_1","unstructured":"\u00a0"},{"key":"e_1_2_7_19_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-022-28381-x"},{"key":"e_1_2_7_20_2","doi-asserted-by":"publisher","DOI":"10.1039\/D2EE02267B"},{"key":"e_1_2_7_21_1","unstructured":"\u00a0"},{"key":"e_1_2_7_22_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-023-38460-2"},{"key":"e_1_2_7_23_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202302583"},{"key":"e_1_2_7_24_1","unstructured":"\u00a0"},{"key":"e_1_2_7_25_2","doi-asserted-by":"publisher","DOI":"10.1039\/D2EE03777G"},{"key":"e_1_2_7_26_2","doi-asserted-by":"publisher","DOI":"10.1021\/acsnano.2c01571"},{"key":"e_1_2_7_27_1","unstructured":"\u00a0"},{"key":"e_1_2_7_28_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.ensm.2022.07.036"},{"key":"e_1_2_7_29_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.3c03030"},{"key":"e_1_2_7_30_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.202300403"},{"key":"e_1_2_7_31_1","unstructured":"\u00a0"},{"key":"e_1_2_7_32_2","doi-asserted-by":"publisher","DOI":"10.1002\/inf2.12374"},{"key":"e_1_2_7_33_2","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202301620"},{"key":"e_1_2_7_34_2","doi-asserted-by":"publisher","DOI":"10.1002\/smll.202003106"},{"key":"e_1_2_7_35_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-26947-9"},{"key":"e_1_2_7_36_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.scib.2022.01.027"},{"key":"e_1_2_7_37_1","doi-asserted-by":"publisher","DOI":"10.1039\/D0TA11841A"},{"key":"e_1_2_7_38_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-018-04060-8"},{"key":"e_1_2_7_39_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202207209"},{"key":"e_1_2_7_40_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2022.06.002"},{"key":"e_1_2_7_41_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsenergylett.3c01017"},{"key":"e_1_2_7_42_1","unstructured":"\u00a0"},{"key":"e_1_2_7_43_2","unstructured":"M.\u2005J. 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