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It also discusses the synthesis, reactivity and catalytic applications of intermolecular, intramolecular and so\u2010called hidden FLPs with phosphorus, nitrogen and carbon Lewis bases. The intrinsically higher acidity of aluminum compounds compared to their boron analogs opens up different reaction pathways. The results are presented in a more or less chronological order. It is shown that Al FLPs react with a variety of polar and non\u2010polar substrates and form both stable adducts and reversibly activate bonds. Consequently, some catalytic applications of the title compounds were presented such as dimerization of alkynes, hydrogenation of <jats:italic>tert<\/jats:italic>\u2010butyl ethylene and imines, C\u2212F bond activation, reduction of CO<jats:sub>2<\/jats:sub>, dehydrogenation of amine borane and transfer of ammonia. 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