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Herein, we demonstrated a photophysical tuning strategy in a new 0D hybrid zinc halide family of (BTPP)\n                    <jats:sub>2<\/jats:sub>\n                    ZnX\n                    <jats:sub>4<\/jats:sub>\n                    (BTPP=benzyltriphenylphosphonium, X=Cl and Br). Infrequently, the delicate combination of organic and inorganic species enables this family to display multiple ultralong green afterglow and efficient self\u2010trapped exciton (STE) associated cyan phosphorescence. Compared with inert luminescence of [BTPP]\n                    <jats:sup>+<\/jats:sup>\n                    cation, incorporation of anionic [ZnX\n                    <jats:sub>4<\/jats:sub>\n                    ]\n                    <jats:sup>2\u2212<\/jats:sup>\n                    effectively enhance the spin\u2010orbit coupling effect, which significantly boosts the photoluminescence quantum yield (PLQY) up to 30.66\u2009% and 54.62\u2009% for afterglow and phosphorescence, respectively. Synchronously, the corresponding luminescence lifetime extend to 143.94\u2005ms and 0.308\u2005\n                    <jats:italic>\u03bc<\/jats:italic>\n                    s surpassing the indiscernible phosphorescence of [BTPP]X salt. More importantly, this halide family presents robust RTP emission with nearly unattenuated PLQY in water and harsh condition (acid and basic aqueous solution) over half a year. The highly efficient integrated afterglow and STE phosphorescence as well as ultrahigh aqueous state RTP realize multiple anti\u2010counterfeiting applications in wide chemical environments.\n                  <\/jats:p>","DOI":"10.1002\/anie.202412350","type":"journal-article","created":{"date-parts":[[2024,8,17]],"date-time":"2024-08-17T05:48:59Z","timestamp":1723873739000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":93,"title":["Synchronously Improved Multiple Afterglow and Phosphorescence Efficiencies in 0D Hybrid Zinc Halides With Ultrahigh Anti\u2010Water Stabilities"],"prefix":"10.1002","volume":"63","author":[{"given":"Jian\u2010Qiang","family":"Zhao","sequence":"first","affiliation":[{"name":"School of Chemistry, Chemical Engineering and Materials Jining University  Qufu Shandong 273155 P. R. 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