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Here, we propose combining DAC with widely used industrial cooling towers to extract CO<jats:sub>2<\/jats:sub> from the air and using electrolysis to release the captured CO<jats:sub>2<\/jats:sub> at room temperature. We first prepare a buffered absorbent solution consisting of sodium glycinate, glycine, and sodium chloride for effective CO<jats:sub>2<\/jats:sub> capture from the air, solving the incompatibility problem of the cooling towers with conventional absorbents. Next, we employ a three\u2010chamber electrolyzer for efficient release (\u226595\u2009%) of the captured CO<jats:sub>2<\/jats:sub> with high purity (\u226598\u2009%) by constant current electrolysis at room temperature, bypassing the conventional energy\u2010intensive heating process. The entire DAC system can operate stably for multiple cycles, and the mechanism for consecutive CO<jats:sub>2<\/jats:sub> capture and release is uncovered. This work reveals the great potential of running DAC in industrial cooling towers coupled with electrochemically\u2010driven CO<jats:sub>2<\/jats:sub> release, opening up new avenues for curbing the increasingly severe climate change.<\/jats:p>","DOI":"10.1002\/anie.202412697","type":"journal-article","created":{"date-parts":[[2024,12,23]],"date-time":"2024-12-23T11:03:38Z","timestamp":1734951818000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["Efficient Direct Air Capture in Industrial Cooling Towers Mediated by Electrochemical CO<sub>2<\/sub> Release"],"prefix":"10.1002","volume":"64","author":[{"given":"Ao\u2010Chuan","family":"Zheng","sequence":"first","affiliation":[{"name":"Environment Research Institute Shandong University  266237 Qingdao China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ye\u2010Bin","family":"Zou","sequence":"additional","affiliation":[{"name":"Environment Research Institute Shandong University  266237 Qingdao China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lin","family":"Du","sequence":"additional","affiliation":[{"name":"Environment Research Institute Shandong University  266237 Qingdao China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qiang","family":"Zhang","sequence":"additional","affiliation":[{"name":"Shandong Lanxiang Environmental Technology Co. 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