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However, the low utilization of the Li source, which suffers from the deteriorated contact interfaces, results in cycling degeneration. Herein, Li\u2212Ag alloy\u2010based artificial electron channels (AECs) are established in Li source\/graphite anode contact interfaces to promote Li\u2010source conversion. Due to the shielding effect of the Li\u2212Ag alloy (50\n                    <jats:italic>at<\/jats:italic>\n                    . % Li) on Li\u2010ion diffusion, the dry\u2010state interfacial corrosion is restricted. The unblocked electronic conduction across the AEC\u2010involved interface not only facilitates the Li\u2010source conversion but also accelerates the prelithiation kinetics during the wet\u2010state process, resulting in an ultrahigh Li\u2010source utilization (90.7\u2009%). Implementing AEC\u2010assisted prelithiation in a LiNi\n                    <jats:sub>0.5<\/jats:sub>\n                    Co\n                    <jats:sub>0.2<\/jats:sub>\n                    Mn\n                    <jats:sub>0.3<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    pouch cell yields a 35.8\u2009% increase in energy density and stable cycling over 600 cycles. This finding affords significant insights into the construction of an efficient prelithiation technology for the development of high\u2010energy LIBs.\n                  <\/jats:p>","DOI":"10.1002\/anie.202413926","type":"journal-article","created":{"date-parts":[[2024,10,2]],"date-time":"2024-10-02T00:28:28Z","timestamp":1727828908000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":42,"title":["Artificial Electron Channels Enable Contact Prelithiation of Li\u2010Ion Battery Anodes with Ultrahigh Li\u2010Source Utilization"],"prefix":"10.1002","volume":"64","author":[{"given":"Xinyang","family":"Yue","sequence":"first","affiliation":[{"name":"Tsinghua Center for Green Chemical Engineering Electrification Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical Engineering Tsinghua University  Beijing 100084 P. R. 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