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All polymers exhibited accumulation mode behavior in OECT devices, and tuning of the donor comonomer resulted in a three\u2010order\u2010of\u2010magnitude increase in transconductance. The best polymer gFBT\u2010g2T, exhibited normalized peak transconductance (\n                    <jats:italic>g<\/jats:italic>\n                    <jats:sub>m,norm<\/jats:sub>\n                    ) of 298\u00b110.4\u2005S\u2009cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    with a corresponding product of charge\u2010carrier mobility and volumetric capacitance,\n                    <jats:italic>\u03bcC<\/jats:italic>\n                    *, of 847\u2009F\u2009V\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u2009cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u2009s\n                    <jats:sup>\u22121<\/jats:sup>\n                    and a\n                    <jats:italic>\u03bc<\/jats:italic>\n                    of 5.76\u2005cm\n                    <jats:sup>2<\/jats:sup>\n                    \u2009V\n                    <jats:sup>\u22121<\/jats:sup>\n                    \u2009s\n                    <jats:sup>\u22121<\/jats:sup>\n                    , amongst the highest reported to date. Furthermore, gFBT\u2010g2T exhibited exceptional temperature stability, maintaining the outstanding electrochemical performance even after undergoing a standard (autoclave) high pressure steam sterilization procedure. Steam treatment was also found to promote film porosity, with the formation of circular 200\u2013400\u2005nm voids. These results demonstrate the potential of gFBT\u2010g2T in p\u2010type accumulation mode OECTs, and pave the way for the use in implantable bioelectronics for medical applications.\n                  <\/jats:p>","DOI":"10.1002\/anie.202416288","type":"journal-article","created":{"date-parts":[[2024,9,18]],"date-time":"2024-09-18T06:21:19Z","timestamp":1726640479000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["High Performance Organic Mixed Ionic\u2010Electronic Polymeric Conductor with Stability to Autoclave Sterilization"],"prefix":"10.1002","volume":"64","author":[{"given":"Hailiang","family":"Liao","sequence":"first","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Achilleas","family":"Savva","sequence":"additional","affiliation":[{"name":"Delft University of Technology Fac. EEMCS  Mekelweg\u20054 2628\u2005CD Delft The Netherlands"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Adam V.","family":"Marsh","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu\u2010Ying","family":"Yang","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hendrik","family":"Faber","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Martina","family":"Rimmele","sequence":"additional","affiliation":[{"name":"Department of Chemistry and Centre for Processable Electronics Imperial College London  W12\u20090BZ London United Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Matteo","family":"Sanviti","sequence":"additional","affiliation":[{"name":"Universidade da Coru\u00f1a Campus Industrial de Ferrol CITENI  Campus Esteiro S\/N 15403 Ferrol Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Renqian","family":"Zhou","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Abdul\u2010Hamid","family":"Emwas","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) KAUST core lab  23955 Thuwal Saudi Arabia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jaime","family":"Mart\u00edn","sequence":"additional","affiliation":[{"name":"Universidade da Coru\u00f1a Campus Industrial de Ferrol CITENI  Campus Esteiro S\/N 15403 Ferrol Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Thomas D.","family":"Anthopoulos","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"},{"name":"Henry Royce Institute and Photon Science Institute Department of Electrical and Electronic Engineering The University of Manchester  Oxford Road M13\u20099PL Manchester United Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6879-5020","authenticated-orcid":false,"given":"Martin","family":"Heeney","sequence":"additional","affiliation":[{"name":"King Abdullah University of Science and Technology (KAUST) Division of Physical Sciences &amp; Engineering  23955 Thuwal Saudi Arabia"},{"name":"Department of Chemistry and Centre for Processable Electronics Imperial College London  W12\u20090BZ London United Kingdom"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,11,2]]},"reference":[{"key":"e_1_2_7_1_1","unstructured":"\u00a0"},{"key":"e_1_2_7_2_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.1c00266"},{"key":"e_1_2_7_3_2","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202101874"},{"key":"e_1_2_7_4_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.6b00146"},{"key":"e_1_2_7_5_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41563-022-01450-8"},{"key":"e_1_2_7_6_2","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202300580"},{"key":"e_1_2_7_7_2","doi-asserted-by":"publisher","DOI":"10.1002\/advs.202306191"},{"key":"e_1_2_7_8_1","unstructured":"\u00a0"},{"key":"e_1_2_7_9_2","doi-asserted-by":"publisher","DOI":"10.1038\/natrevmats.2017.86"},{"key":"e_1_2_7_10_2","doi-asserted-by":"publisher","DOI":"10.1021\/acsaelm.1c00312"},{"key":"e_1_2_7_11_2","volume":"30","author":"Sun H.","year":"2018","journal-title":"Adv. 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