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Photomagnetic behavior is often observed in spin transition materials, including spin\u2010crossover complexes, and can lead to long\u2010range magnetic ordering. Photo\u2010induced magnetization can affect different physical properties, including second harmonic generation. Still, despite a growing number of luminescent spin\u2010crossover systems, the simultaneous switching of both magnetism and luminescence was not yet explored. In this regard, we present systematic studies for a novel coordination polymer composed of anionic Nd\n                    <jats:sup>III<\/jats:sup>\n                    \u2013[W\n                    <jats:sup>IV<\/jats:sup>\n                    (CN)\n                    <jats:sub>8<\/jats:sub>\n                    ]\n                    <jats:sup>4\u2013<\/jats:sup>\n                    layers, crystallizing with chiral organic cations embedded in the interlayer space. Not only we observe and rationalize theoretically near\u2010infrared emission of Nd\n                    <jats:sup>III<\/jats:sup>\n                    centers sensitized by [W\n                    <jats:sup>IV<\/jats:sup>\n                    (CN)\n                    <jats:sub>8<\/jats:sub>\n                    ]\n                    <jats:sup>4\u2013<\/jats:sup>\n                    units, but we also found a plausible pathway to track the photomagnetic effect throughout the analysis of the Nd\n                    <jats:sup>3+<\/jats:sup>\n                    excitation spectra and their temperature dependence. The observed thermally reversible effects in luminescence were correlated with the results of photomagnetic studies, providing an attractive pathway to monitor the light\u2010induced magnetization changes through a photoluminescent read\u2010out.\n                  <\/jats:p>","DOI":"10.1002\/anie.202424651","type":"journal-article","created":{"date-parts":[[2025,4,22]],"date-time":"2025-04-22T04:45:27Z","timestamp":1745297127000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["Luminescent Detection of Photomagnetic Effect in a Near\u2010Infrared Emissive Neodymium(III)\u2013Octacyanidotungstate(IV) Framework"],"prefix":"10.1002","volume":"64","author":[{"given":"Jakub J.","family":"Zakrzewski","sequence":"first","affiliation":[{"name":"Faculty of Chemistry Jagiellonian University in Krak\u00f3w  Gronostajowa 2 Krak\u00f3w 30\u2013387 Poland"},{"name":"Doctoral School of Exact and Natural Sciences Jagiellonian 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