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Herein reported single\u2010crystal X\u2010ray diffraction studies reveal an acetylide type [ArC{N(Dipp)}(Dipp)NC\u2261CLi)]\n                    <jats:sub>\n                      <jats:italic>n<\/jats:italic>\n                    <\/jats:sub>\n                    (\n                    <jats:bold>3<\/jats:bold>\n                    \u2010Ar) dimeric (\n                    <jats:italic>n<\/jats:italic>\n                    = 2) or trimeric (\n                    <jats:italic>n<\/jats:italic>\n                    = 3) molecular structure for\n                    <jats:bold>2<\/jats:bold>\n                    \u2010Ar. Treatment of\n                    <jats:bold>3<\/jats:bold>\n                    \u2010Ph with Et\n                    <jats:sub>3<\/jats:sub>\n                    B cleanly yields the monoanionic carbene Li[(ADC)(BEt\n                    <jats:sub>3<\/jats:sub>\n                    )] (\n                    <jats:bold>4<\/jats:bold>\n                    \u2010Ph) featuring a weakly coordinating anion embedded in the same molecular entity.\n                    <jats:bold>3<\/jats:bold>\n                    \u2010Ar readily undergo reactions with CO\n                    <jats:sub>2<\/jats:sub>\n                    and N\n                    <jats:sub>2<\/jats:sub>\n                    O to form the ring\u2010closing products Li[(ADC)(CO\n                    <jats:sub>2<\/jats:sub>\n                    )\n                    <jats:sub>2<\/jats:sub>\n                    ] (\n                    <jats:bold>5<\/jats:bold>\n                    \u2010Ar) and Li[(ADC)N\n                    <jats:sub>2<\/jats:sub>\n                    O] (\n                    <jats:bold>6<\/jats:bold>\n                    \u2010Ar), respectively.\n                  <\/jats:p>","DOI":"10.1002\/anie.202501068","type":"journal-article","created":{"date-parts":[[2025,3,11]],"date-time":"2025-03-11T08:18:39Z","timestamp":1741681119000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":10,"title":["Lithium Anionic Dicarbenes or Acetylides: What is in the Name?"],"prefix":"10.1002","volume":"64","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-8788-7200","authenticated-orcid":false,"given":"Arne","family":"Merschel","sequence":"first","affiliation":[{"name":"Molecular Inorganic Chemistry and Catalysis Inorganic and Structural Chemistry Center for Molecular Materials Faculty of Chemistry Universit\u00e4t Bielefeld  Universit\u00e4tsstrasse\u200525 D-33615 Bielefeld Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5187-2242","authenticated-orcid":false,"given":"Henric","family":"Steffenfauseweh","sequence":"additional","affiliation":[{"name":"Molecular Inorganic Chemistry and Catalysis Inorganic and Structural Chemistry Center for Molecular Materials Faculty of Chemistry Universit\u00e4t Bielefeld  Universit\u00e4tsstrasse\u200525 D-33615 Bielefeld Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-7130-6280","authenticated-orcid":false,"given":"Yury V.","family":"Vishnevskiy","sequence":"additional","affiliation":[{"name":"Molecular Inorganic Chemistry and Catalysis Inorganic and Structural Chemistry Center for Molecular Materials Faculty of Chemistry Universit\u00e4t Bielefeld  Universit\u00e4tsstrasse\u200525 D-33615 Bielefeld Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Beate","family":"Neumann","sequence":"additional","affiliation":[{"name":"Molecular Inorganic Chemistry and Catalysis Inorganic and Structural Chemistry Center for Molecular Materials Faculty of Chemistry Universit\u00e4t Bielefeld  Universit\u00e4tsstrasse\u200525 D-33615 Bielefeld Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hans\u2010Georg","family":"Stammler","sequence":"additional","affiliation":[{"name":"Molecular Inorganic Chemistry and Catalysis Inorganic and Structural Chemistry Center for Molecular Materials Faculty of Chemistry Universit\u00e4t Bielefeld  Universit\u00e4tsstrasse\u200525 D-33615 Bielefeld Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2146-5432","authenticated-orcid":false,"given":"Rajendra S.","family":"Ghadwal","sequence":"additional","affiliation":[{"name":"Molecular Inorganic Chemistry and Catalysis Inorganic and Structural Chemistry Center for Molecular Materials Faculty of Chemistry Universit\u00e4t Bielefeld  Universit\u00e4tsstrasse\u200525 D-33615 Bielefeld Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,3,11]]},"reference":[{"key":"e_1_2_8_1_1","unstructured":"\u00a0"},{"key":"e_1_2_8_2_2","doi-asserted-by":"publisher","DOI":"10.1002\/zaac.201700394"},{"key":"e_1_2_8_3_2","doi-asserted-by":"publisher","DOI":"10.1039\/C4DT01004C"},{"key":"e_1_2_8_4_2","doi-asserted-by":"crossref","unstructured":"F. 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