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Traditional SEI layers are limited by their simple structure and composition, enabling only one functionality of either providing nucleation sites or facilitating desolvation. In this study, a pulse guidance ion\u2010accelerator is constructed by kinetics\u2010controlled co\u2010assembly of zincophilic micelles and zincophobic metal\u2010organic framework (MOF). The closely packed soft micelles, in conjunction with the hard MOF host particles, form a multi\u2010tiered soft\u2010in\u2010hard hetero\u2010structure that accelerates adsorption, pre\u2010desolvation, and subsequent desolvation processes, facilitating the (002) crystal plane dendrite\u2010free deposition. As a result, stable cycling over 1900 h (31\u00a0mV polarization) in symmetric cell and 5200 cycles in the Zn\/\/Cu battery (99.8% coulombic efficiency) can be achieved. 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