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The prepared TAT\u2010AZO\u2010COF with three\u2010motif molecular junction units, resulting from the integration of a cathode\u2010active carbonyl group, an anode\u2010active azo group, and a changeably bipolar\u2010active triazin group, could provide a tunable voltage inductive effect to simultaneously meet the requirements of SAOBs. Thus\u2010assembled SAOBs display excellent rate performance, high energy density (125\u00a0Wh kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    ) at 1 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    and superior long\u2010cycle property (90 mAh g\n                    <jats:sup>\u22121<\/jats:sup>\n                    over 10\u00a0000 cycles) at 10 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , which is represented to be the best high\u2010current density performance among all the organic electrode materials in dual\u2010electrode available SAOBs. The Li\n                    <jats:sup>+<\/jats:sup>\n                    storage mechanisms of three\u2010motif molecular junction COFs are thoroughly scrutinized by experimental and theoretical identification, and the feasibility in practical application has been validated by a successfully assembled pouch cell.\n                  <\/jats:p>","DOI":"10.1002\/anie.202508937","type":"journal-article","created":{"date-parts":[[2025,5,28]],"date-time":"2025-05-28T22:26:54Z","timestamp":1748471214000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["Three\u2010Motif Molecular Junction Covalent Organic Frameworks for Symmetric All\u2010Organic Lithium\u2010Ion Battery"],"prefix":"10.1002","volume":"64","author":[{"given":"Wenhai","family":"Feng","sequence":"first","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University  Guangzhou 510006 P.R. 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China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhengyang","family":"Chen","sequence":"additional","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University  Guangzhou 510006 P.R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1718-6871","authenticated-orcid":false,"given":"Yifa","family":"Chen","sequence":"additional","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University  Guangzhou 510006 P.R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ya\u2010Qian","family":"Lan","sequence":"additional","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University  Guangzhou 510006 P.R. China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2025,6,3]]},"reference":[{"key":"e_1_2_9_1_1","doi-asserted-by":"publisher","DOI":"10.1007\/s41918-022-00135-9"},{"key":"e_1_2_9_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.progpolymsci.2021.101449"},{"key":"e_1_2_9_3_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41578-022-00478-1"},{"key":"e_1_2_9_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ensm.2020.12.027"},{"key":"e_1_2_9_5_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.202102693"},{"key":"e_1_2_9_6_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2020.10.028"},{"key":"e_1_2_9_7_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.202200912"},{"key":"e_1_2_9_8_1","doi-asserted-by":"publisher","DOI":"10.1002\/adma.200803073"},{"key":"e_1_2_9_9_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201501780"},{"key":"e_1_2_9_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201901040"},{"key":"e_1_2_9_11_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jpowsour.2013.07.007"},{"key":"e_1_2_9_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2022.139016"},{"key":"e_1_2_9_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.nanoen.2021.106055"},{"key":"e_1_2_9_14_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202207221"},{"key":"e_1_2_9_15_1","doi-asserted-by":"publisher","DOI":"10.1039\/D1TA06228J"},{"key":"e_1_2_9_16_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202317135"},{"key":"e_1_2_9_17_1","doi-asserted-by":"publisher","DOI":"10.1002\/aenm.201703509"},{"key":"e_1_2_9_18_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202113315"},{"key":"e_1_2_9_19_1","doi-asserted-by":"publisher","DOI":"10.1021\/acsnano.3c11780"},{"key":"e_1_2_9_20_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202210871"},{"key":"e_1_2_9_21_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202207043"},{"key":"e_1_2_9_22_1","first-page":"354","volume":"41","author":"An Y.","year":"2021","journal-title":"Energy Environ. 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