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Herein, a novel acceptor BMD\u20106F was synthesized via molecular engineering of L8\u2010BO, which realizes synergistic optimization of dielectric constant (6.20, 1.5 \u00d7 that of L8\u2010BO) and H\u2010aggregation and thus enriches charge transport pathways, facilitates exciton dissociation, and suppresses recombination. As a result, the PM6:L8\u2010BO:BMD\u20106F ternary OSC delivered a champion PCE of 20.34% at 100\u00a0nm, and exhibited excellent thickness tolerance with PCEs of 18.23% (300\u00a0nm) and 16.18% (500\u00a0nm). This work establishes a design principle for high\u2010efficiency, thickness\u2010tolerant OSCs, promising industrial applications.<\/jats:p>","DOI":"10.1002\/anie.2077291","type":"journal-article","created":{"date-parts":[[2026,10,12]],"date-time":"2026-10-12T02:25:09Z","timestamp":1791771909000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Synergistic Regulation of High Dielectric Constant and H\u2010Aggregation for Efficient and Thickness\u2010Tolerant Organic Solar Cells"],"prefix":"10.1002","author":[{"given":"Peng","family":"Zhang","sequence":"first","affiliation":[{"name":"College of Chemistry Key Laboratory of Advanced Green Functional Materials Changchun Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yunhan","family":"Gao","sequence":"additional","affiliation":[{"name":"Key Laboratory of Automobile Materials Ministry of Education, and School of Materials Science and Engineering Jilin University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0003-7967-1607","authenticated-orcid":false,"given":"Linsen","family":"Li","sequence":"additional","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shuai","family":"Xu","sequence":"additional","affiliation":[{"name":"College of Chemistry Key Laboratory of Advanced Green Functional Materials Changchun Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shuhan","family":"Yang","sequence":"additional","affiliation":[{"name":"College of Chemistry Key Laboratory of Advanced Green Functional Materials Changchun Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7061-6781","authenticated-orcid":false,"given":"Youdi","family":"Zhang","sequence":"additional","affiliation":[{"name":"College of Chemistry Key Laboratory of Advanced Green Functional Materials Changchun Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7364-3312","authenticated-orcid":false,"given":"Meifang","family":"Zhang","sequence":"additional","affiliation":[{"name":"Institute of Carbon Neutral New Energy School of Intelligent Materials and New Energy Yuzhang Normal University  Nanchang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nan","family":"Ye","sequence":"additional","affiliation":[{"name":"College of Chemistry Key Laboratory of Advanced Green Functional Materials Changchun Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lixue","family":"Zhu","sequence":"additional","affiliation":[{"name":"College of Chemistry Key Laboratory of Advanced Green Functional Materials Changchun Normal University  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0006-3231-5885","authenticated-orcid":false,"given":"Tao","family":"Jia","sequence":"additional","affiliation":[{"name":"Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5496-5858","authenticated-orcid":false,"given":"Sha","family":"Liu","sequence":"additional","affiliation":[{"name":"Dongguan Key Laboratory of Interdisciplinary Science For Advanced Materials and Large\u2010Scale Scientific Facilities School of Physical Sciences Great Bay University  Dongguan Guangdong China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8484-7249","authenticated-orcid":false,"given":"Zicheng","family":"Ding","sequence":"additional","affiliation":[{"name":"Shaanxi Key Laboratory For Advanced Energy Devices Shaanxi Engineering Lab For Advanced Energy Technology School of Materials Science and Engineering Shaanxi Normal University  Xi'an China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-3951-1484","authenticated-orcid":false,"given":"Hongxiang","family":"Li","sequence":"additional","affiliation":[{"name":"College of Materials and Energy Guang'an Institute of Technology  Guang'an Sichuan P. 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