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Cobalt\u2010catalyzed metal\u2013hydride hydrogen atom transfer (Co\u2500H\/MHAT) has emerged as a powerful platform for alkene hydroamination by enabling the controlled generation of carbon\u2010centered radicals under mild and near\u2010neutral conditions. This review summarizes the development of Co\u2013MHAT\u2010enabled C\u2500N bond formation from its origins to recent advances, tracing all transformations to a common Co\u2500H\u2010initiated radical\/organocobalt branch point. Across both reductive Co\/photoredox and oxidative Co\u2013MHAT manifolds, a common Co\u2500H\u2010initiated step generates a shared radical\/organocobalt intermediate that can be directed into distinct pathways, including radical\u2013radical coupling (RRC), radical\u2013polar crossover (RPC), and radical ligand transfer (RLT). These complementary reactivity modes enable amination at sterically hindered and electronically unbiased sites. Collectively, Co\u2013MHAT catalysis offers a versatile and conceptually distinct strategy for selective C\u2500N bond construction.<\/jats:p>","DOI":"10.1002\/anie.3165931","type":"journal-article","created":{"date-parts":[[2026,9,18]],"date-time":"2026-09-18T13:57:17Z","timestamp":1789739837000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Cobalt\u2010Catalyzed C\u2500N Bond Formation via Metal\u2010Hydride Hydrogen Atom Transfer (MHAT)"],"prefix":"10.1002","author":[{"ORCID":"https:\/\/orcid.org\/0009-0000-6768-7132","authenticated-orcid":false,"given":"Arman","family":"Khosravi","sequence":"first","affiliation":[{"name":"James Tarpo Jr. and Margaret Tarpo Department of Chemistry Purdue University  West Lafayette Indiana United 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