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Here, we design a dual\u2010engine catalytic system for CO\n                    <jats:sub>2<\/jats:sub>\n                    hydrogenation to aromatics via a synergistic C\n                    <jats:sub>2+<\/jats:sub>\n                    alcohols\/olefins pathway. The dual\u2010engine catalytic system initiated by FeCo active sites and CuZnAl promoters guarantees the continuous C\n                    <jats:sub>2+<\/jats:sub>\n                    alcohols\/olefins supply, delivering a record\u2010breaking aromatics yield (31.1%) with the aid of aromatization component H\u2010ZSM\u20105. Multiple characterization and theoretical simulations reveal that C\n                    <jats:sub>2+<\/jats:sub>\n                    alcohols trigger carbon\u2010chain growth through oxonium\u2010mediated rapid carbocation generation via a low\u2010barrier \u201cprotonation\u2010dehydration\u201d sequence, whereas olefins serve as \u03c0\u2010substrates to propagate carbon\u2010chain. This synergy accelerates both oligomerization and subsequent aromatization, effectively circumventing both the sluggish initial C\u2500C coupling of methanol\u2010mediated pathways and the high\u2010barrier direct protonation step in olefins\u2010mediated pathways. Techno\u2010economic analysis (TEA) further demonstrates the superior industrial viability of this novel process. This work establishes a new paradigm for designing efficient catalytic systems and engineering process toward sustainable CO\n                    <jats:sub>2<\/jats:sub>\n                    valorization.\n                  <\/jats:p>","DOI":"10.1002\/anie.3604576","type":"journal-article","created":{"date-parts":[[2026,7,3]],"date-time":"2026-07-03T17:36:06Z","timestamp":1783100166000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["A Synergistic C\n                    <sub>2+<\/sub>\n                    Alcohols\/Olefins\u2010Intermediated Pathway Boosts CO\n                    <sub>2<\/sub>\n                    Hydrogenation to Aromatics"],"prefix":"10.1002","volume":"65","author":[{"given":"Xinze","family":"Bi","sequence":"first","affiliation":[{"name":"College of New Energy China University of Petroleum (East China)  Qingdao China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qi","family":"Li","sequence":"additional","affiliation":[{"name":"College of New Energy China University of Petroleum (East China)  Qingdao China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Na","family":"Zhao","sequence":"additional","affiliation":[{"name":"Wison Engineering Services Co. 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