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Strategically, constructing bimetallic pairs with asymmetric active sites is a key strategy for further improving DACs performances. However, achieving the universal synthesis of a structurally controllable library for DACs supported on inorganic materials remains a significant challenge. In this work, we propose a general strategy for synthesizing asymmetric DACs (A\u2010DACs) through molecular explosion, which can transiently generate extreme conditions in a confined space, offering capabilities that are difficult to realize by conventional approaches. Using this technology, we successfully prepared and systematically characterized 15 kinds of\n                    <jats:italic>A<\/jats:italic>\n                    \u2010DACs containing different metal combinations (Cu\u2010Fe, Cu\u2010Co, Fe\u2010Pt, Ni\u2010Cu, Pt\u2010Pd etc.) and loaded them onto different inorganic carriers (Ti\n                    <jats:sub>3<\/jats:sub>\n                    C\n                    <jats:sub>2<\/jats:sub>\n                    T\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    , TiN, TiO\n                    <jats:sub>2<\/jats:sub>\n                    , CeO\n                    <jats:sub>2<\/jats:sub>\n                    , MoS\n                    <jats:sub>2<\/jats:sub>\n                    , etc.). Moreover, Cu\n                    <jats:sub>1<\/jats:sub>\n                    Fe\n                    <jats:sub>1<\/jats:sub>\n                    \/Ti\n                    <jats:sub>3<\/jats:sub>\n                    C\n                    <jats:sub>2<\/jats:sub>\n                    T\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    and Pt\n                    <jats:sub>1<\/jats:sub>\n                    Pd\n                    <jats:sub>1<\/jats:sub>\n                    \/MoS\n                    <jats:sub>2<\/jats:sub>\n                    are selected as model catalysts to investigate their worthwhile applications in diverse electrochemical reactions. This study provides an ingenious method for the rational design of atomic dispersed catalysts, which is of great significance in the fields of energy conversion and environmental governance scenarios.\n                  <\/jats:p>","DOI":"10.1002\/anie.3998491","type":"journal-article","created":{"date-parts":[[2026,6,11]],"date-time":"2026-06-11T07:56:22Z","timestamp":1781164582000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Dual Atom Catalysts Through Explosion"],"prefix":"10.1002","volume":"65","author":[{"given":"Zihao","family":"Wei","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Beijing Institute of Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhiyi","family":"Sun","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Beijing Institute of Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xilin","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Physics Henan Normal University  Xinxiang China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qian","family":"Bai","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Beijing Institute of Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Huilong","family":"Geng","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Beijing Institute of Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziheng","family":"Zhan","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Beijing Institute of Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yan","family":"Gao","sequence":"additional","affiliation":[{"name":"Anhui Provincial Engineering Research Center of Silicon\u2010based Materials Bengbu University  Bengbu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0864-5124","authenticated-orcid":false,"given":"Huan","family":"Wang","sequence":"additional","affiliation":[{"name":"School of Chemistry and Chemical Engineering Center For Interdisciplinary Health Management Studies Guangzhou Key Laboratory of Sensing Materials &amp; Devices Guangzhou University  Guangzhou China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qi","family":"Sun","sequence":"additional","affiliation":[{"name":"School of Materials Science and Engineering Beijing Institute of Technology  Beijing China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Fang","family":"Zhang","sequence":"additional","affiliation":[{"name":"Experimental Center of Advanced Materials Beijing Institute of Technology  Beijing P. 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