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We report a donor glycolated, quinoidal design that facilitates efficient n\u2010doping and spatially separates hydrophilic side chains from n\u2010doping sites to preserve electronic pathways. The resulting polymer PQ\u2010gT, synthesized from a glycolated bithiophene donor and a quinoidal bifuran\u2010dione acceptor, exhibits high mixed conduction with a figure of merit of\n                    <jats:italic>\u00b5C<\/jats:italic>\n                    * = 10.9 F cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    V\n                    <jats:sup>\u22121<\/jats:sup>\n                    s\n                    <jats:sup>\u22121<\/jats:sup>\n                    . In planar accumulation\u2010mode organic electrochemical transistors (OECTs), it exhibits nearly symmetric sub\u2010millisecond transients with switching on\u2010 and off\u2010times of\n                    <jats:italic>\u03c4<\/jats:italic>\n                    <jats:sub>on<\/jats:sub>\n                    \/\n                    <jats:italic>\u03c4<\/jats:italic>\n                    <jats:sub>off<\/jats:sub>\n                    = 0.5\/0.2\u00a0ms. These values represent the fastest operation for this type of device architecture. Partial donor replacement with dialkoxybithiazole tunes packing and suppresses swelling, raising\n                    <jats:italic>\u00b5C<\/jats:italic>\n                    * to 21.5 F cm\n                    <jats:sup>\u22121<\/jats:sup>\n                    V\n                    <jats:sup>\u22121<\/jats:sup>\n                    s\n                    <jats:sup>\u22121<\/jats:sup>\n                    at 25% substitution, albeit with slower switching. In vertical OECTs, PQ\u2010gT supports balanced ambipolar operation with \u223c1\u00a0ms switching and enables a single\u2010material complementary inverter (gain \u2248 40\u00a0V V\n                    <jats:sup>\u22121<\/jats:sup>\n                    at V\n                    <jats:sub>IN<\/jats:sub>\n                    &lt; 100\u00a0mV) that is stable over 10\u00a0000 cycles and functional up to 200\u00a0Hz. This donor\u2010glycolated quinoidal strategy furnishes intrinsically fast, aqueous\u2010stable n\u2010type organic mixed ionic\u2010electronic conductors for bioelectronic circuits.\n                  <\/jats:p>","DOI":"10.1002\/anie.4114731","type":"journal-article","created":{"date-parts":[[2026,8,12]],"date-time":"2026-08-12T17:07:53Z","timestamp":1786554473000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Donor\u2010Glycolated Quinoidal Polymers Enable Fast N\u2010Type Organic Electrochemical Transistors"],"prefix":"10.1002","volume":"65","author":[{"given":"Jun","family":"Zhang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Polymer Science and Technology Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun China"},{"name":"School of Applied Chemistry and Engineering University of Science and Technology of China  Hefei 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Chengdu China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1522-634X","authenticated-orcid":false,"given":"Zhongxiang","family":"Peng","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Polymer Science and Technology Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiaocong","family":"Zhou","sequence":"additional","affiliation":[{"name":"Institute of Molecular Aggregation Science Tianjin University  Tianjin China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hangyang","family":"Li","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Polymer Science and Technology Changchun Institute of Applied Chemistry Chinese Academy of Sciences  Changchun China"},{"name":"School of Applied Chemistry and Engineering University of Science and Technology of China  Hefei 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