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However, their intrinsic trade\u2010off between large dissymmetry factor and high carrier mobility (\n                    <jats:italic>\u03bc<\/jats:italic>\n                    ) hinders the application for high\u2010performance CPL detection. To overcome this issue, the chiral induction combined with the ring\u2010fusion strategy is employed to rationally construct a new n\u2010type chiral nanographene imide (\n                    <jats:italic>S<\/jats:italic>\n                    )\u2010Cy\u2010FT\u2010FPDI. In the monomeric state, (\n                    <jats:italic>S<\/jats:italic>\n                    )\u2010Cy\u2010FT\u2010FPDI exhibited distinct circular dichroism (CD) signals, with the maximum absorption dissymmetry factor (\n                    <jats:italic>g<\/jats:italic>\n                    <jats:sub>abs<\/jats:sub>\n                    ) reaching \u22122.16 \u00d7 10\n                    <jats:sup>\u22123<\/jats:sup>\n                    . The (\n                    <jats:italic>S<\/jats:italic>\n                    )\u2010Cy\u2010FT\u2010FPDI annealed thin films presented dual\u2010wavelength CPL responses at 455 and 595\u00a0nm, with photocurrent dissymmetry factors (\n                    <jats:italic>g<\/jats:italic>\n                    <jats:sub>ph<\/jats:sub>\n                    ) of 0.22 and 0.53, respectively, while delivering high\n                    <jats:italic>\u03bc<\/jats:italic>\n                    of 0.57\u00a0cm\n                    <jats:sup>2<\/jats:sup>\n                    V\n                    <jats:sup>\u22121<\/jats:sup>\n                    s\n                    <jats:sup>\u22121<\/jats:sup>\n                    , successfully balancing the favorable electrical performance and excellent chiroptical property. Remarkably, the achieved\n                    <jats:italic>\u03bc<\/jats:italic>\n                    and\n                    <jats:italic>g<\/jats:italic>\n                    <jats:sub>ph<\/jats:sub>\n                    outperform most of the previously reported chiral organic small\u2010molecule counterparts. Then, we have successfully demonstrated the high\u2010fidelity encoding and encryption based on (\n                    <jats:italic>S<\/jats:italic>\n                    )\u2010Cy\u2010FT\u2010FPDI annealed thin films. Our work provides a feasible molecular design strategy for chiral organic small molecules with concurrent high\n                    <jats:italic>g<\/jats:italic>\n                    <jats:sub>ph<\/jats:sub>\n                    and\n                    <jats:italic>\u03bc<\/jats:italic>\n                    , balancing\u00a0the dissymmetry factor\u2010mobility trade\u2010off towards high\u2010performance CPL detection.\n                  <\/jats:p>","DOI":"10.1002\/anie.4944869","type":"journal-article","created":{"date-parts":[[2026,10,24]],"date-time":"2026-10-24T07:08:27Z","timestamp":1792825707000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Chiral Nanographene Imides: Balancing the Dissymmetry Factor\u2010Mobility Trade\u2010Off Towards Circularly Polarization\u2010Sensitive Photodetection"],"prefix":"10.1002","author":[{"given":"Jinhang","family":"Liu","sequence":"first","affiliation":[{"name":"State Key Laboratory for Porous Metal Materials School of Materials Science and Engineering Xi'an Jiaotong University  Xi'an People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chao","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Bioinspired Interfacial Materials Science Suzhou Institute for Advanced Research University of Science and Technology of China  Suzhou Jiangsu People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenkai","family":"Zhao","sequence":"additional","affiliation":[{"name":"Frontiers Science Center for New Organic Matter Tianjin Key Lab for Rare Earth Materials and Applications Renewable Energy Conversion and Storage Center (RECAST) Academy for Advanced Interdisciplinary Studies School of Materials Science and Engineering Nankai University  Tianjin People's Republic of 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