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Existing approaches typically focus on individual optimization of each electrode, limiting full cell to achieve synergistic enhancement and inevitably increases system complexity. Herein, a dual\u2010affinity three\u2010dimensional host is constructed by integrating one\u2010dimensional carbon nanotubes with two\u2010dimensional vermiculite nanosheets. The incorporation of vermiculite overcomes the intrinsically low polarity and weak adsorption capability with active material of the conventional 3D carbon frameworks. Benefiting from the densely stacked hybrid architecture with high mechanical strength, excellent electrical conductivity and dual affinity toward Zn and polyiodides, the 3D host concurrent regulate Zn deposition and iodine conversion chemistry. The zincophilic vermiculite regulate Zn\n                    <jats:sup>2+<\/jats:sup>\n                    flux, lower the nucleation barrier and promote uniform deposition, while the porous structure effectively suppress polyiodide shuttling through synergistic physical confinement and chemical anchoring. Consequently, the Zn composite anode exhibits remarkable cycling stability over 3000 cycles at 20\u00a0mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    at 60% depth\u2010of\u2010discharge, whereas the integrated Zn\u2010I\n                    <jats:sub>2<\/jats:sub>\n                    full cell maintains 90.0% capacity retention after 2000 cycles. This work offers a route for designing durable, highly efficient Zn\u2010I\n                    <jats:sub>2<\/jats:sub>\n                    batteries.\n                  <\/jats:p>","DOI":"10.1002\/anie.5243975","type":"journal-article","created":{"date-parts":[[2026,9,2]],"date-time":"2026-09-02T11:11:21Z","timestamp":1788347481000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Dual\u2010Affinity Host Engineering for Highly Reversible Zinc\u2013Iodine Batteries"],"prefix":"10.1002","volume":"65","author":[{"given":"Meijia","family":"Chen","sequence":"first","affiliation":[{"name":"School of Chemistry and Materials Science Jiangsu Normal University  Xuzhou Jiangsu P.R China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0000-8760-2757","authenticated-orcid":false,"given":"Chuang","family":"Sun","sequence":"additional","affiliation":[{"name":"College of Chemical and 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