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Supramolecular organic weaves offer many benefits, such as error correction, but their functionalization is challenging, as even minor modifications to the building blocks can disrupt self\u2010assembly. In this study, we demonstrate that a triaxially woven supramolecular organic framework formed by the self\u2010assembly of an oligoproline\u2013perylene monoimide conjugate tolerates pre\u2010assembly functionalization and enables homogeneous incorporation of acetyl, pivaloyl, and thiophene moieties without altering the woven structure. Thiophene functionalization enabled the binding of toxic and noble\u2010metal ions from aqueous solution within the weave's confined pores. These results establish first examples of functionalized supramolecular organic weaves and highlight the value of modular peptide\u2010based woven frameworks for targeted guest encapsulation.<\/jats:p>","DOI":"10.1002\/anie.5300884","type":"journal-article","created":{"date-parts":[[2026,9,26]],"date-time":"2026-09-26T12:14:38Z","timestamp":1790424878000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Functionalization and Metal Ion Encapsulation Within a Triaxial Supramolecular Weave"],"prefix":"10.1002","author":[{"given":"Andreas","family":"Herdlitschka","sequence":"first","affiliation":[{"name":"Laboratory of Organic Chemistry D\u2010CHAB ETH Zurich Zurich Switzerland"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tatiana","family":"Da Silva\u2010Ferreira","sequence":"additional","affiliation":[{"name":"Laboratory of Organic Chemistry D\u2010CHAB ETH Zurich Zurich 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