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However, the simultaneous electroreduction construction of C\u2500C and C\u2500N bonds is challenging. Herein, we propose a strategy to construct C\u2500C and C\u2500N bonds in tandem at the cathode and anode, respectively. At the cathode, a nitrate\u2010induced dynamic Cu\n                    <jats:sup>\u03b4+<\/jats:sup>\n                    site is designed to promote C\u2500C coupling activity from CO\n                    <jats:sub>2<\/jats:sub>\n                    reduction to ethanol, which is accompanied by the generation of ammonia from nitrate reduction, with a total Faradaic efficiency of 88.6%. The generated ethanol and ammonia serve as feedstocks for the tandem construction of C\u2500N bonds at the anodic region via a possible nucleophilic attack pathway. We achieve the synthesis of acetamide with a Faradaic efficiency of 71.4% and a yield rate of 0.13\u00a0mmol h\n                    <jats:sup>\u22121<\/jats:sup>\n                    cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . The carbon footprint analysis of this tandem strategy revealed net\u2010zero emissions at a carbon intensity of 0.23 kg\n                    <jats:sub>CO2e<\/jats:sub>\n                    kWh\n                    <jats:sup>\u22121<\/jats:sup>\n                    , indicating its sustainable nature from the viewpoint of carbon neutrality.\n                  <\/jats:p>","DOI":"10.1002\/anie.5526884","type":"journal-article","created":{"date-parts":[[2026,5,23]],"date-time":"2026-05-23T11:37:13Z","timestamp":1779536233000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["Nitrate\u2010Stabilized Cu\n                    <sup>\u03b4+<\/sup>\n                    Sites Promote Selective CO\n                    <sub>2<\/sub>\n                    Electroreduction to Ethanol for Tandem Acetamide 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