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Here, we report a ligand\u2010protected strategy to simultaneously encapsulate subnanometric CeO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    and Pt clusters within silicalite\u20101 (S\u20101) zeolite. Zeolite confinement stabilizes both Pt and CeO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    species under reducing dehydrogenation conditions, while the dynamic and reversible formation of strong Pt\u2013CeO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    interactions facilitates the reversible redispersion of Pt species during oxidative regeneration. Notably, the Pt\u20104CeO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    @S\u20101 catalyst remains fully regenerable after 9 consecutive redox cycles and sustained operation over 5000\u00a0min at 600\u00b0C. Even after steam treatment at 600\u00b0C, the catalyst fully recovers its activity through simple calcination\u2013reduction, demonstrating outstanding structural durability under industrially relevant conditions. Integrated theoretical and experimental evidence shows that confinement within the zeolite framework allows CeO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    to dynamically capture mobile PtO\n                    <jats:italic>\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    via Pt\u2013O\u2012Ce bond formation, facilitating atomic\u2010scale Pt redispersion under oxidative conditions. This work offers a generalizable strategy for constructing redox\u2010adaptive catalyst architectures with built\u2010in self\u2010regeneration, advancing the design of robust zeolite\u2010based catalysts for high\u2010temperature and cyclic catalytic processes.\n                  <\/jats:p>","DOI":"10.1002\/anie.5533379","type":"journal-article","created":{"date-parts":[[2026,5,18]],"date-time":"2026-05-18T15:39:51Z","timestamp":1779118791000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Built\u2010In Self\u2010Regeneration of Platinum Catalysis in Propane Dehydrogenation with Rare\u2010Earth\u2010Modified Zeolites"],"prefix":"10.1002","volume":"65","author":[{"given":"Liwen","family":"Guo","sequence":"first","affiliation":[{"name":"Innovation Center for Chemical Science College of Chemistry Chemical Engineering and Materials Science Jiangsu Key Laboratory of Advanced Negative Carbon Technologies Soochow 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