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In this work, we demonstrate the impressive afterglow of commercial benzene\u2010carboxylic acid (BCA) derivatives are attributed to trace impurities identified as biphenyl carboxylic acid derivatives. One of the impurities even induces detectable phosphorescence when the doping ratio is\u00a0as low as 0.1\u00a0ppm (molar ratio). Inspired by the structural similarity between impurities and the main component, we propose a pseudo\u2010homologues strategy for constructing afterglow materials. Based on this model, several groups of compounds are used to prepare 275 doped samples. Surprisingly, pseudo\u2010homologues exhibit a markedly higher success rate for afterglow (73.3%) compared to that of other samples (6.5%). 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