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Herein, we propose a concept of molecular structure entropy for the development of a high\u2010entropy polymer (HEP), wherein molecular structure entropy exerts a significant regulatory effect on the physicochemical and electrochemical performance of the resulting polymer. For sodium\u2010based batteries, the Na||HEP cell delivers a high reversible capacity of 167.7\u00a0mAh\u00a0g\n                    <jats:sup>\u22121<\/jats:sup>\n                    at a current density of 1\u00a0A\u00a0g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , a long cycling stability of 5000 cycles, and a high\u2010rate capability of 111.9\u00a0mAh\u00a0g\n                    <jats:sup>\u22121<\/jats:sup>\n                    at a current density of 10\u00a0A\u00a0g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , outperforming the low\u2010entropy polymer. Moreover, the all\u2010organic battery shows a long stability of 15\u00a0000 cycles, corresponding to a continuous running time exceeding 200 days. This work sets a precedent for HEP electrodes and establishes a foundation for their further research.\n                  <\/jats:p>","DOI":"10.1002\/anie.6867886","type":"journal-article","created":{"date-parts":[[2026,5,23]],"date-time":"2026-05-23T12:14:46Z","timestamp":1779538486000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":3,"title":["High\u2010Entropy Polymer Electrode for Fast Rechargeable Batteries"],"prefix":"10.1002","volume":"65","author":[{"given":"Yanyao","family":"Hu","sequence":"first","affiliation":[{"name":"College of Materials and Energy Central South University of Forestry and Technology  Changsha People's Republic of China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4813-3895","authenticated-orcid":false,"given":"Ling","family":"Fan","sequence":"additional","affiliation":[{"name":"School of Physics and Electronics Hunan University  Changsha People's 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