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However, the lack of mastery over reconstruction kinetics typically imposes a trade\u2010off between high activity and long\u2010term stability. Here, we demonstrate that the degree of chemical ordering (long\u2010range atomic site occupancy) deterministically governs the evolution of alloy surfaces under operating conditions. In this design, the chemical ordering acts as a structural template that commands the reconstruction trajectory. During anodic dealloying, the ordered lattice facilitates a controlled, mild pre\u2010oxidation. This process generates high\u2010valence Fe\/Co\/Ni sites that trigger a well\u2010balanced, synergistic adsorbate evolution mechanism (AEM)\/lattice oxygen mechanism (LOM) dual pathway. Unlike disordered counterparts that suffer from severe deterioration, the thermodynamically stable intermetallic core prevents excessive metal dissolution, reducing elemental leaching by 97.2%, guiding the formation of a homogeneous active reconstruction layer. As a result, the catalyst achieves an overpotential of only 335\u00a0mV at 1 A cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    and maintains exceptional stability for over 1000\u00a0h. Even under industrial conditions (6\u00a0M KOH, 353 K), it reaches 3 A cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    at only 1.50\u00a0V. This work establishes chemical ordering as a predictive parameter to govern dynamic reconstruction, offering a robust framework for designing self\u2010adaptive catalysts that harmonize extreme activity with industrial\u2010grade durability.\n                  <\/jats:p>","DOI":"10.1002\/anie.6881208","type":"journal-article","created":{"date-parts":[[2026,7,23]],"date-time":"2026-07-23T10:51:23Z","timestamp":1784803883000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Chemical Ordering Command Dynamic Reconstruction for Enhanced Water Oxidation"],"prefix":"10.1002","volume":"65","author":[{"given":"Yiyuan","family":"Yang","sequence":"first","affiliation":[{"name":"School of Materials Science and Engineering Southeast University Nanjing China"},{"name":"Department of Mechanical Engineering City University of Hong Kong Hong Kong China"},{"name":"Hong Kong Branch of National Precious Metals Material Engineering 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