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However, their markedly different thermodynamic profiles have precluded their simultaneous incorporation into a single polymer. Here we report a novel reaction strategy for the selective construction of formal CO\/CO\n                    <jats:sub>2<\/jats:sub>\n                    \/butadiene terpolymers in a 1:1:2 molar ratio. This protocol involves the Pd\u2010catalyzed telomerization of CO\n                    <jats:sub>2<\/jats:sub>\n                    with butadiene to form a lactone\u2010based intermediate (EVP), followed by its catalytic alternating copolymerization with CO, affording functional polyketones bearing pendent unsaturated lactone side groups in high yields. Notably, both the ketone and lactone functionalities within the functional polymers can be quantitatively reduced to hydroxyl groups using sodium borohydride (NaBH\n                    <jats:sub>4<\/jats:sub>\n                    ) at room temperature. The obtained multi\u2010hydroxy functionalized polymer exhibits strong adhesion to common substrates (adhesion strength up to 10.13\u00a0MPa on wood) together with desirable oxidative degradability.\n                  <\/jats:p>","DOI":"10.1002\/anie.6906738","type":"journal-article","created":{"date-parts":[[2026,3,8]],"date-time":"2026-03-08T09:19:26Z","timestamp":1772961566000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Functional Polymer Synthesis From CO, CO\n                    <sub>2<\/sub>\n                    , and Butadiene"],"prefix":"10.1002","volume":"65","author":[{"given":"Fulin","family":"Zhou","sequence":"first","affiliation":[{"name":"Frontiers Science Center For Transformative Molecules Shanghai Key Laboratory For Molecular Engineering of Chiral Drugs School of Chemistry and Chemical Engineering Shanghai Jiao Tong University  Shanghai 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