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Here we engineer an epitaxially stabilized CuO overlayer on Ti\n                    <jats:sub>1\u2010x<\/jats:sub>\n                    In\n                    <jats:sub>x<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    that breaks the activity\u2013selectivity\u2013stability constraint by creating electron\u2010poor, high\u2010symmetry Cu\u2013O sites and activating lattice\u2010oxygen redox at the oxide\u2013oxide interface. Interfacial strain and charge transfer increase Cu\u2013O covalency and Lewis acidity, accelerating NO\n                    <jats:sub>x<\/jats:sub>\n                    reduction via an Eley\u2013Rideal pathway while diverting sulfate deposition away from Cu. Concurrently, interface\u2010activated lattice oxygen sustains deep oxidation of CH\n                    <jats:sub>3<\/jats:sub>\n                    SH (a representative S\u2010VOC) through a Mars\u2013van Krevelen cycle, suppressing HCN. Epitaxial interfaces thus offer a general route to poison\u2010resistant multipollutant catalysis.\n                  <\/jats:p>","DOI":"10.1002\/anie.7111765","type":"journal-article","created":{"date-parts":[[2026,8,12]],"date-time":"2026-08-12T17:01:57Z","timestamp":1786554117000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Epitaxial Oxide Interfaces Create Poison\u2010Resistant CuO Sites for Environmental Catalysis"],"prefix":"10.1002","volume":"65","author":[{"ORCID":"https:\/\/orcid.org\/0009-0000-7690-5832","authenticated-orcid":false,"given":"Lupeng","family":"Han","sequence":"first","affiliation":[{"name":"International Joint Laboratory of Catalytic Chemistry State Key Laboratory of Materials for Advanced Nuclear Energy Innovation Institute of Carbon Neutrality Department of Chemistry College of Sciences Shanghai University  Shanghai People's Republic of 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