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For organic scintillators, employing triplet excitons represents a useful strategy to increase the radioluminescence intensity. However, utilization of the triplet excitons generally conflicts with the development of fast scintillators, which are key to fast\u2010timing medical radiography. Here, we design a series of efficient fluorophores with anti\u2010Kasha energy levels, enabling fast scintillation by effectively utilizing high\u2010lying triplet excitons. As a result, the fluorescent scintillators exhibit short lifetimes in the nanosecond range and a low detection limit of 21.7 nGy s\n                    <jats:sup>\u22121<\/jats:sup>\n                    , which is two orders of magnitude lower than the dosage for x\u2010ray medical diagnostics. Encouraged by the results, we further employ high\u2010throughput virtual screening to accelerate the development of fast organic scintillators and demonstrate their potential in advanced radiography. This design principle could provide inspirations to exploit efficient fast organic scintillators, thereby advancing the applications of organic scintillators in the x\u2010ray community.\n                  <\/jats:p>","DOI":"10.1002\/anie.7669745","type":"journal-article","created":{"date-parts":[[2026,8,20]],"date-time":"2026-08-20T12:04:43Z","timestamp":1787227483000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Efficient Organic Fluorescence Scintillation by Engineering Anti\u2010Kasha Triplet Energy Levels"],"prefix":"10.1002","volume":"65","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-6021-4938","authenticated-orcid":false,"given":"Xiao","family":"Wang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Flexible Electronics (LoFE) &amp; Institute of Advanced Materials (IAM) School of Flexible Electronics (Future Technologies) Nanjing Tech University (NanjingTech)  Nanjing 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