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Herein, we report a new Zr\u2010MOF (PCN\u20101010), featuring a\n                    <jats:bold>scu<\/jats:bold>\n                    topology with channel\u2010type porosity via ligand conformational bending. Distinct from the\n                    <jats:bold>ftw<\/jats:bold>\n                    \u2010topology Zr\u2010MOF with cage\u2010type porosity constructed from a straight tetra\u2010topic ligand, PCN\u20101010 contains 8\u2010connected Zr\n                    <jats:sub>6<\/jats:sub>\n                    clusters with more accessible catalytic sites and open one\u2010dimensional (1D) channels. The bent conformation of the linker creates alternating concave and convex surfaces along the\n                    <jats:italic>c<\/jats:italic>\n                    \u2010axis, facilitating the accessibility of the active sites. In addition, PCN\u20101010 exhibits high chemical stability in various organic solvents owing to the robust zirconium\u2010oxo coordination. As a catalytic platform for sulfide oxidation, PCN\u20101010, integrated with 12\u2010tungstophosphoric acid, delivers high\u2010selectivity sulfone production with a yield of 97% instead of sulfoxide at room temperature, alongside good recyclability and broad substrate compatibility. The enhanced catalytic performance of PCN\u20101010 relative to its cage\u2010type\n                    <jats:bold>ftw<\/jats:bold>\n                    counterpart demonstrates that rational pore geometry regulation via ligand bending is an effective route to optimize mass transport and active\u2010site accessibility.\n                  <\/jats:p>","DOI":"10.1002\/anie.7849352","type":"journal-article","created":{"date-parts":[[2026,10,22]],"date-time":"2026-10-22T04:03:55Z","timestamp":1792641835000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Tuning Pore Geometry of Zirconium Metal\u2013Organic Frameworks via Bent Ligands for Enhanced Sulfide Oxidation Catalysis"],"prefix":"10.1002","author":[{"given":"Zhaoyi","family":"Liu","sequence":"first","affiliation":[{"name":"Department of Chemistry Texas A&amp;M University  College Station Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0002-5701-1547","authenticated-orcid":false,"given":"Joshua","family":"Rushlow","sequence":"additional","affiliation":[{"name":"Department of Chemistry Texas A&amp;M University  College Station Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0000-6446-1728","authenticated-orcid":false,"given":"Jiatong","family":"Huo","sequence":"additional","affiliation":[{"name":"Department of Chemistry Texas A&amp;M University  College Station Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wenlu","family":"Fan","sequence":"additional","affiliation":[{"name":"Department of Chemistry University of North Texas  Denton Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kui","family":"Tan","sequence":"additional","affiliation":[{"name":"Department of Chemistry and Biochemistry The University of Texas at El Paso  El Paso Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1897-7069","authenticated-orcid":false,"given":"Shengqian","family":"Ma","sequence":"additional","affiliation":[{"name":"Department of Chemistry University of North Texas  Denton Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5356-9928","authenticated-orcid":false,"given":"Rong\u2010Ran","family":"Liang","sequence":"additional","affiliation":[{"name":"Department of Chemistry Texas A&amp;M University  College Station Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9029-3788","authenticated-orcid":false,"given":"Hong\u2010Cai","family":"Zhou","sequence":"additional","affiliation":[{"name":"Department of Chemistry Texas A&amp;M University  College Station Texas USA"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2026,10,21]]},"reference":[{"key":"e_1_2_8_2_1","doi-asserted-by":"crossref","first-page":"1342","DOI":"10.1038\/s41557-022-01093-x","article-title":"Merging Molecular Catalysts and Metal\u2013Organic Frameworks for Photocatalytic Fuel Production","volume":"14","author":"Stanley P. 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