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However, challenges like the polyiodide shuttle effect, sluggish conversion kinetics, and Zn dendrite growth hinder their practical application. Herein, we reported to design \u2018ship\u2010in\u2010bottle\u2019 structured polyiodide electrocatalyst to simultaneously prevent the shuttle effect and promote the catalytic conversion of polyiodides. The implanted ultrafine Ag nanoparticles inside the carbonaceous framework can offer potent active centres to confine the I\n                    <jats:sup>\u2212<\/jats:sup>\n                    and facilitate the I\n                    <jats:sup>\u2212<\/jats:sup>\n                    \/I\n                    <jats:sub>2<\/jats:sub>\n                    conversion through the adsorption of I\n                    <jats:sup>\u2212<\/jats:sup>\n                    by forming AgI. Meanwhile, the generated AgI further contributes to anchoring the polyiodides, effectively suppressing its shuttle effect. The strong hybridization between Ag\n                    <jats:italic>d<\/jats:italic>\n                    orbitals and iodine\n                    <jats:italic>p<\/jats:italic>\n                    orbitals enables efficient charge transfer during conversion. Therefore, the Zn\u2010I\n                    <jats:sub>2<\/jats:sub>\n                    \u00a0battery exhibits high discharge capacity over 200 mAh g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , excellent rate capability up to 10 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    , and long\u2010term cycling stability (30 000 cycles at 6 A g\n                    <jats:sup>\u22121<\/jats:sup>\n                    ). The practicality is also validated via pouch cell with impressive energy density of 180\u00a0Wh kg\n                    <jats:sup>\u22121<\/jats:sup>\n                    based on the cathode and excellent cycling stability over 500 cycles, enlightening the material engineering for catalyst design towards rapid polyiodide conversion. Our findings offer valuable guidance for the development of high\u2010performance Zn\u2010I\n                    <jats:sub>2<\/jats:sub>\n                    batteries.\n                  <\/jats:p>","DOI":"10.1002\/anie.8096588","type":"journal-article","created":{"date-parts":[[2026,5,22]],"date-time":"2026-05-22T13:29:33Z","timestamp":1779456573000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Iodide Anion Anchoring by Silver Nanoparticles Enables Shuttle\u2010Free Zinc\u2010Iodine Batteries"],"prefix":"10.1002","volume":"65","author":[{"given":"Lichao","family":"Tan","sequence":"first","affiliation":[{"name":"Institute of Carbon Neutrality Zhejiang Wanli University  Ningbo China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shaojian","family":"Zhang","sequence":"additional","affiliation":[{"name":"School of Chemical Engineering The University of Adelaide Adelaide 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