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While surface\u2010assisted assembly of symmetric, non\u2010interacting DNA origami nanostructures offers a facile route to 2D superlattices, existing approaches typically yield close\u2010packed arrays with limited control over inter\u2010origami spacing. Here, we present a tunable and reproducible strategy for regulating the lateral spacing of DNA origami during self\u2010assembly into macroscopic 2D lattice patterns. By controlling the growth of uniform single\u2010stranded polynucleotide brushes from the surface of DNA origami, we modulate their effective geometry by introducing longer\u2010ranged entropic repulsion, which enables precise and adjustable control over inter\u2010origami distances across macroscopic areas. Using integrated experiments and simulations, we demonstrate how systematic variation of brush length, surface adsorption strength, and brush density can lead to tunable surface patterns across different origami shapes. Overall, this straightforward approach advances the field of DNA\u2010templated nanofabrication by providing highly programmable templates with precise spatial control. This platform offers a robust foundation for the future integration of functional nanomaterials and the development of organized nanostructures.<\/jats:p>","DOI":"10.1002\/anie.8367703","type":"journal-article","created":{"date-parts":[[2026,6,4]],"date-time":"2026-06-04T08:53:04Z","timestamp":1780563184000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Tunable Patterning of DNA Origami on Surfaces Using Steric Brushes"],"prefix":"10.1002","volume":"65","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-4681-3886","authenticated-orcid":false,"given":"Shuang","family":"Wang","sequence":"first","affiliation":[{"name":"State Key Laboratory of Marine Food Processing &amp; Safety Control Laboratory For Marine Drugs and Bioproducts Qingdao Marine Science and Technology Center College of Food Science and Engineering Ocean University of China  Qingdao China"},{"name":"Wallace H. Coulter Department of Biomedical Engineering Georgia Institute of Technology and Emory University  Atlanta Georgia USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5235-3807","authenticated-orcid":false,"given":"Po\u2010An","family":"Lin","sequence":"additional","affiliation":[{"name":"Thomas Lord Department of Mechanical Engineering and Materials Science Duke University  Durham North Carolina USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2290-7178","authenticated-orcid":false,"given":"Stefan","family":"Zauscher","sequence":"additional","affiliation":[{"name":"Thomas Lord Department of Mechanical Engineering and Materials Science Duke University  Durham North Carolina USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5615-0521","authenticated-orcid":false,"given":"Gaurav","family":"Arya","sequence":"additional","affiliation":[{"name":"Thomas Lord Department of Mechanical Engineering and Materials Science Duke University  Durham North Carolina USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1673-2153","authenticated-orcid":false,"given":"Yonggang","family":"Ke","sequence":"additional","affiliation":[{"name":"Wallace H. Coulter Department of Biomedical Engineering Georgia Institute of Technology and Emory University  Atlanta Georgia 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