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However, practical methods for fabricating such complex morphologies remain limited. Here, we demonstrate an instantaneous mechanically driven strategy for simultaneously programming particle shape and surface architecture through a refined rubbing process. By optimizing particle plasticization, pressure distribution, and stress transmission, spherical polymer particles were transformed into cylindrical particles within only 10 s. Patterned silicon substrates enabled direct mechanical transfer of periodic surface structures, while variations in substrate topology and deformation pathway produced diverse anisotropic architectures. This simple mechanically driven process provides a straightforward platform for programming hierarchical polymer microparticle architectures.<\/jats:p>","DOI":"10.1002\/anie.8528979","type":"journal-article","created":{"date-parts":[[2026,9,30]],"date-time":"2026-09-30T05:22:46Z","timestamp":1790745766000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Instantaneous Mechanical Programming of Polymer Microparticle Shape and Surface Architecture"],"prefix":"10.1002","author":[{"given":"Tomoki","family":"Nakagami","sequence":"first","affiliation":[{"name":"Department of Chemical Science and Engineering Graduate School of Engineering Kobe University, Rokko, Nada  Kobe Japan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1914-5686","authenticated-orcid":false,"given":"Akihide","family":"Arima","sequence":"additional","affiliation":[{"name":"Research Institute for Quantum 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