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However, for catalytic reactions that present decoupled rate\u2010 and selectivity\u2010limiting steps, the alloying site density may significantly manipulate these independent steps, but it has rarely been explicitly examined for any SAA systems. Herein, using the electrocatalytic CO reduction as a probe reaction, we report that the nominal Pd\n                    <jats:sub>1<\/jats:sub>\n                    Cu cube\u00a0SAA catalysts exhibit distinctive high reactivity toward ethylene or ethanol, respectively, depending on whether the Pd atoms are in dilute or crowded forms.\u00a0Although the presence of single\u2010atom Pd embedded on Cu uniformly promotes CHO* formation and C\u2500C coupling, the dilute\u2010Pd\n                    <jats:sub>1<\/jats:sub>\n                    Cu favors ethylene formation by enabling low\u2010barrier C\u2500O cleavage from a flat CH\n                    <jats:sub>2<\/jats:sub>\n                    CH\n                    <jats:sub>2<\/jats:sub>\n                    OH* intermediate, whereas the crowded\u2010Pd\n                    <jats:sub>1<\/jats:sub>\n                    Cu promotes ethanol formation by stabilizing an upright hydrogenation transition state of the same intermediate. Furthermore, we present evidence that the catalytic chemistry of crowded Pd\n                    <jats:sub>1<\/jats:sub>\n                    \u00a0species differs from that of the Pd\n                    <jats:sub>2<\/jats:sub>\n                    \u2010dimer; the latter, albeit unstable, steers reaction selectivity to acetate instead. These results uncovered the underappreciated importance of controlling SAA catalytic chemistry from the perspective of single\u2010atom site densities.\n                  <\/jats:p>","DOI":"10.1002\/anie.9720330","type":"journal-article","created":{"date-parts":[[2026,6,1]],"date-time":"2026-06-01T08:07:37Z","timestamp":1780301257000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Variations of Alloying Site Density in Pd\n                    <sub>1<\/sub>\n                    Cu Single\u2010Atom Alloy Catalysts Lead to Shifted Product Yields in Electrochemical CO Reduction"],"prefix":"10.1002","volume":"65","author":[{"given":"Zehua","family":"Jin","sequence":"first","affiliation":[{"name":"Department of Chemical and Biomolecular Engineering Clemson University  Clemson South Carolina USA"},{"name":"Zhejiang Key Laboratory of Extreme Environment Functional Materials Yiwu Research Institute of Fudan University  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