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Its versatile catalytic activity arises exclusively due to the presence of a non\u2010innocent ligand, which can trigger its unique redox properties effectively. These complexes have been employed widely in (transfer)hydrogenation (e.\u2009g., reduction of polar multiple bonds, Oppenauer\u2010type oxidation of alcohols), C\u2212C and C\u2212N bond formation (e.\u2009g., reductive aminations, <jats:italic>\u03b1<\/jats:italic>\u2010alkylation of ketones) and other synthetic transformations. In this review, we discuss the remarkable advancement of its various synthetic applications along with synthesis and mechanistic studies, until February 2021.<\/jats:p>","DOI":"10.1002\/asia.202100400","type":"journal-article","created":{"date-parts":[[2021,5,17]],"date-time":"2021-05-17T11:51:55Z","timestamp":1621252315000},"page":"1703-1724","update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":36,"title":["(Cyclopentadienone)iron Complexes: Synthesis, Mechanism and Applications in Organic Synthesis"],"prefix":"10.1002","volume":"16","author":[{"given":"Monalisa","family":"Akter","sequence":"first","affiliation":[{"name":"Department of Chemistry Indian Institute of Technology Madras  Chennai 600036 India"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6049-5023","authenticated-orcid":false,"given":"Pazhamalai","family":"Anbarasan","sequence":"additional","affiliation":[{"name":"Department of Chemistry Indian Institute of Technology Madras  Chennai 600036 India"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2021,6]]},"reference":[{"key":"e_1_2_12_1_1","doi-asserted-by":"publisher","DOI":"10.1021\/cr500425u"},{"key":"e_1_2_12_2_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.8b00372"},{"key":"e_1_2_12_3_1","doi-asserted-by":"publisher","DOI":"10.1021\/cr300236r"},{"key":"e_1_2_12_4_1","doi-asserted-by":"publisher","DOI":"10.1039\/c0cc05733a"},{"key":"e_1_2_12_5_1","doi-asserted-by":"publisher","DOI":"10.1039\/C7CY00879A"},{"key":"e_1_2_12_6_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.200301553"},{"key":"e_1_2_12_6_2","doi-asserted-by":"publisher","DOI":"10.1002\/ange.200301553"},{"key":"e_1_2_12_7_1","doi-asserted-by":"publisher","DOI":"10.1021\/acscentsci.6b00272"},{"key":"e_1_2_12_8_1","doi-asserted-by":"publisher","DOI":"10.1039\/b612251e"},{"key":"e_1_2_12_9_1","doi-asserted-by":"publisher","DOI":"10.1126\/science.1183281"},{"key":"e_1_2_12_10_1","doi-asserted-by":"publisher","DOI":"10.1002\/ejic.201100985"},{"key":"e_1_2_12_11_1","doi-asserted-by":"publisher","DOI":"10.1021\/cs200660v"},{"key":"e_1_2_12_12_1","doi-asserted-by":"publisher","DOI":"10.1039\/C2CS35228A"},{"key":"e_1_2_12_13_1","doi-asserted-by":"publisher","DOI":"10.1039\/C4CC90480J"},{"key":"e_1_2_12_14_1","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.9b03337"},{"key":"e_1_2_12_15_1","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201310788"},{"key":"e_1_2_12_15_2","doi-asserted-by":"publisher","DOI":"10.1002\/ange.201310788"},{"key":"e_1_2_12_16_1","doi-asserted-by":"publisher","DOI":"10.1002\/ejoc.201901925"},{"key":"e_1_2_12_17_1","doi-asserted-by":"publisher","DOI":"10.1055\/s-2004-831293"},{"key":"e_1_2_12_18_1","doi-asserted-by":"publisher","DOI":"10.1021\/cr9003133"},{"key":"e_1_2_12_19_1","doi-asserted-by":"publisher","DOI":"10.1021\/om00127a027"},{"key":"e_1_2_12_20_1","doi-asserted-by":"publisher","DOI":"10.1021\/ja00283a041"},{"key":"e_1_2_12_21_1","doi-asserted-by":"publisher","DOI":"10.1002\/jlac.19535820107"},{"key":"e_1_2_12_22_1","doi-asserted-by":"publisher","DOI":"10.1021\/ja01623a092"},{"key":"e_1_2_12_23_1","doi-asserted-by":"publisher","DOI":"10.1021\/ja01601a064"},{"key":"e_1_2_12_24_1","first-page":"4020","author":"Jones E. 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