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This work reports the direct growth of Fe\n                    <jats:sup>3+<\/jats:sup>\n                    \/benzene di\u2010carboxylate MOFs onto functionalized silicon surfaces, compatible with a wide range of MOF synthesis conditions. The co\u2010nucleation and growth of different crystalline phases are evidenced, whose coverage depends on the surface chemistry and\/or the solution composition. Three structural phases \u2013 the cubic MIL\u2010101(Fe), a hexagonal phase with a structure close to MOF\u2010235 and a MIL\u201053(Fe) with a monoclinic symmetry \u2010 are identified through characteristic crystal shapes and their structural parameters inferred from X\u2010Ray Diffraction. In addition to the oriented growth of 3D crystallites, the formation of two\u2010dimensional MIL\u2010101 nano\u2010crystallites or thin layers\/islands exhibiting extended monocrystalline domains with (111) texture is also demonstrated through high\u2010resolution atomic force microscopy. Post\u2010synthesis treatments reveal a weak adhesion of the hexagonal phase, indicating a different surface anchoring.\n                  <\/jats:p>","DOI":"10.1002\/asia.202200129","type":"journal-article","created":{"date-parts":[[2022,4,26]],"date-time":"2022-04-26T13:27:21Z","timestamp":1650979641000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":11,"title":["Growth of Fe\u2010BDC Metal\u2010Organic Frameworks onto Functionalized Si (111) Surfaces"],"prefix":"10.1002","volume":"17","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-2997-7793","authenticated-orcid":false,"given":"Hongye","family":"Yuan","sequence":"first","affiliation":[{"name":"Laboratoire de Physique de la Mati\u00e8re Condens\u00e9e CNRS Ecole Polytechnique Institut Polytechnique de Paris  91120 Palaiseau France"},{"name":"Present address: State Key Laboratory for Mechanical Behavior of Materials Shaanxi International Research Center for Soft Matter School of Materials Science and Engineering Xi'an Jiaotong University  Xi'an 710049 P. 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