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Aided by balanced intermolecular \u03c0\u2010\u03c0 interactions, the gelator was capable of gelate pure chloroform and mixed solutions containing chloroform. Interestingly, introducing long hexyl chains in the gelator's structure makes it lose the gelation ability, indicating that alkyl chain is not always favorable auxiliary group for gelation. The gel network was selectively responsive to aniline, which was manifested by aniline\u2010triggered gel collapse. Notably, the gel exhibited remarkable fluorescence blue\u2010shift upon exposure to aniline, rather than quenching, exhibiting ratiometric fluorescence response. The selective response to aniline was due to that aniline could break the original intermolecular \u03c0\u2010\u03c0 interactions in the gel state, providing a unique example of ratiometric gel sensor for aniline.<\/jats:p>","DOI":"10.1002\/asia.202401277","type":"journal-article","created":{"date-parts":[[2025,3,4]],"date-time":"2025-03-04T03:32:26Z","timestamp":1741059146000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Fluorescent Non\u2010conventional D\u2010\u03c0\u2010A Organogel for Aniline Sensing"],"prefix":"10.1002","volume":"20","author":[{"given":"Shuzhan","family":"Chen","sequence":"first","affiliation":[{"name":"College of Materials &amp; Chemical Engineering China Three Gorges University  Yichang Hubei 443002 PR China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Aoran","family":"Sun","sequence":"additional","affiliation":[{"name":"College of Materials &amp; Chemical Engineering China Three Gorges University  Yichang Hubei 443002 PR China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guisheng","family":"Lai","sequence":"additional","affiliation":[{"name":"College of Materials &amp; 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