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Hydrogels were prepared through graft\u2010copolymerization of acrylic acid on cellulose in the presence of ammonium persulfate as initiator, followed by crosslinking with N,<jats:italic>N<\/jats:italic>\u2032\u2010methylenebisacrylamide. The characterization of components, structure, and properties of the rind extract and the hydrogels was carried out. The solvent mixture of water:ethanol 1:2 (v\/v) was the most suitable solvent for the extraction of mangosteen rind. The silver nanoparticle was found to form a strong interaction with the composition of the hydrogel, which resulted in the improvement of the thermal property and the sterilization of both gram\u2010positive and gram\u2010negative bacteria. 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