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Thus, the syntheses and structural analysis of molecular adducts <jats:bold>1\u2009a<\/jats:bold>\u2013<jats:bold>1\u2009c<\/jats:bold> (<jats:bold>1<\/jats:bold> with bpyee, bpyea, and bpy, respectively) and <jats:bold>2\u2009a<\/jats:bold>\u2013<jats:bold>2\u2009c<\/jats:bold> (<jats:bold>2<\/jats:bold> with bpyee, bpyea, and bpy, respectively) are discussed. In all these adducts, recognition between the constituents is established through either O\uf8ffH\u22c5\u22c5\u22c5N and\/or O\uf8ffH\u22c5\u22c5\u22c5N\/C\uf8ffH\u22c5\u22c5\u22c5O pairwise hydrogen bonds. In all the adducts both OH and COOH functional groups available on <jats:bold>1<\/jats:bold> and <jats:bold>2<\/jats:bold> interact with the N\u2010donor compounds, except in <jats:bold>2\u2009a<\/jats:bold>, in which only COOH (COO<jats:sup>\u2212<\/jats:sup>) is involved in the recognition process. The COOH moieties in <jats:bold>1\u2009a<\/jats:bold>, <jats:bold>1\u2009b<\/jats:bold>, and <jats:bold>2\u2009b<\/jats:bold> form only single O\uf8ffH\u22c5\u22c5\u22c5N hydrogen bonds, whereas in <jats:bold>1\u2009c<\/jats:bold> and <jats:bold>2\u2009c<\/jats:bold>, they form pairwise O\uf8ffH\u22c5\u22c5\u22c5N\/C\uf8ffH\u22c5\u22c5\u22c5O hydrogen bonds. In addition, subtle differences in the recognition patterns resulted in the formation of cyclic networks of different dimensions. In fact, only <jats:bold>1\u2009c<\/jats:bold> forms a four\u2010molecule cyclic moiety, as was already documented in the literature for this kind of assemblies. All complexes have been characterized by single\u2010crystal X\u2010ray diffraction. The supramolecular architectures are quite elegant and simple, with stacking of sheets in all adducts, but a rather complex network with a threefold interpenetration pattern was found in <jats:bold>2\u2009c<\/jats:bold>.<\/jats:p>","DOI":"10.1002\/chem.200500570","type":"journal-article","created":{"date-parts":[[2005,10,26]],"date-time":"2005-10-26T03:46:50Z","timestamp":1130298410000},"page":"1597-1609","source":"Crossref","is-referenced-by-count":79,"title":["A Competitive Molecular Recognition Study: Syntheses and Analysis of Supramolecular Assemblies of 3,5\u2010Dihydroxybenzoic Acid and Its Bromo Derivative with Some N\u2010Donor Compounds"],"prefix":"10.1002","volume":"12","author":[{"given":"Sunil","family":"Varughese","sequence":"first","affiliation":[],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Venkateswara 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