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These compounds are of the [Cd(dpm)<jats:sub>2<\/jats:sub>] type, with the coordination sphere of the metal centre occupied by two dpm chelates. Interestingly, in contrast to what has been reported for the Zn<jats:sup>II<\/jats:sup> analogues, in the presence of a pyridyl\u2010 or imidazolyl\u2010appended dpm ligand, the coordination number of the Cd<jats:sup>II<\/jats:sup> cation can be increased to six, leading to an octahedral coordination sphere. As a consequence, the formation of 1\u2010, 2\u2010, and 3D coordination polymers by self\u2010assembly is observed. 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