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Due to the different electronic situations of phosphorus and nitrogen with respect to s and p character of the lone pair, different reactivity of the phosphorus compounds was observed, especially with regard to the specificity of the reactions and the stability of the products. Whereas Mes*N\uf8fePCl (Mes*=2,4,6\u2010tri\u2010<jats:italic>tert<\/jats:italic>\u2010butylphenyl) is stable in the solid state and in solution, the formal phosphorus congener Mes*P\uf8fePCl is highly reactive and could not be observed. 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