{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,19]],"date-time":"2026-08-19T01:26:24Z","timestamp":1787102784287,"version":"build-2736575974"},"reference-count":159,"publisher":"Wiley","issue":"47","license":[{"start":{"date-parts":[[2014,10,3]],"date-time":"2014-10-03T00:00:00Z","timestamp":1412294400000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/onlinelibrary.wiley.com\/termsAndConditions#vor"}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Chemistry A European J"],"published-print":{"date-parts":[[2014,11,17]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>\n                    A study of the scope and limitations of varying the ligand framework around the dinuclear core of FvRu\n                    <jats:sub>2<\/jats:sub>\n                    in its function as a molecular solar thermal energy storage framework is presented. It includes DFT calculations probing the effect of substituents, other metals, and CO exchange for other ligands on \u0394\n                    <jats:italic>H<\/jats:italic>\n                    <jats:sub>storage<\/jats:sub>\n                    . Experimentally, the system is shown to be robust in as much as it tolerates a number of variations, except for the identity of the metal and certain substitution patterns. Failures include 1,1\u2032,3,3\u2032\u2010tetra\u2010\n                    <jats:italic>tert<\/jats:italic>\n                    \u2010butyl (\n                    <jats:bold>4<\/jats:bold>\n                    ), 1,2,2\u2032,3\u2032\u2010tetraphenyl (\n                    <jats:bold>9<\/jats:bold>\n                    ), diiron (\n                    <jats:bold>28<\/jats:bold>\n                    ), diosmium (\n                    <jats:bold>24<\/jats:bold>\n                    ), mixed iron\u2010ruthenium (\n                    <jats:bold>27<\/jats:bold>\n                    ), dimolybdenum (\n                    <jats:bold>29<\/jats:bold>\n                    ), and ditungsten (\n                    <jats:bold>30<\/jats:bold>\n                    ) derivatives. An extensive screen of potential catalysts for the thermal reversal identified AgNO\n                    <jats:sub>3<\/jats:sub>\n                    \u2013SiO\n                    <jats:sub>2<\/jats:sub>\n                    as a good candidate, although catalyst decomposition remains a challenge.\n                  <\/jats:p>","DOI":"10.1002\/chem.201404170","type":"journal-article","created":{"date-parts":[[2014,10,3]],"date-time":"2014-10-03T12:13:30Z","timestamp":1412338410000},"page":"15587-15604","source":"Crossref","is-referenced-by-count":53,"title":["Exploring the Potential of Fulvalene Dimetals as Platforms for Molecular Solar Thermal Energy Storage: Computations, Syntheses, Structures, Kinetics, and Catalysis"],"prefix":"10.1002","volume":"20","author":[{"given":"Karl","family":"B\u00f6rjesson","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Du\u0161an","family":"\u0106oso","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Victor","family":"Gray","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jeffrey C.","family":"Grossman","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jingqi","family":"Guan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Charles B.","family":"Harris","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Norbert","family":"Hertkorn","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zongrui","family":"Hou","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yosuke","family":"Kanai","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Donghwa","family":"Lee","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Justin P.","family":"Lomont","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Arun","family":"Majumdar","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Steven K.","family":"Meier","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Kasper","family":"Moth\u2010Poulsen","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Randy L.","family":"Myrabo","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Son C.","family":"Nguyen","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Rachel A.","family":"Segalman","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Varadharajan","family":"Srinivasan","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Willam B.","family":"Tolman","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Nikolai","family":"Vinokurov","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"K. Peter C.","family":"Vollhardt","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Timothy W.","family":"Weidman","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2014,10,3]]},"reference":[{"key":"e_1_2_6_1_2","unstructured":"For a perspective see:"},{"key":"e_1_2_6_2_2","doi-asserted-by":"publisher","DOI":"10.1126\/science.1218761"},{"key":"e_1_2_6_3_2","doi-asserted-by":"publisher","DOI":"10.1039\/c1ee01861b"},{"key":"e_1_2_6_4_2","doi-asserted-by":"publisher","DOI":"10.1038\/nchem.1918"},{"key":"e_1_2_6_5_2","doi-asserted-by":"publisher","DOI":"10.1021\/jz301877n"},{"key":"e_1_2_6_6_2","doi-asserted-by":"publisher","DOI":"10.1063\/1.4773306"},{"key":"e_1_2_6_7_2","unstructured":"\u00a0"},{"key":"e_1_2_6_8_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.jfluchem.2014.01.012"},{"key":"e_1_2_6_9_2","doi-asserted-by":"publisher","DOI":"10.1039\/c3cp51292d"},{"key":"e_1_2_6_10_2","doi-asserted-by":"publisher","DOI":"10.1039\/c3ta12002c"},{"key":"e_1_2_6_11_2","doi-asserted-by":"publisher","DOI":"10.1021\/sc300107z"},{"key":"e_1_2_6_12_2","doi-asserted-by":"publisher","DOI":"10.1039\/c2ee22426g"},{"key":"e_1_2_6_13_2","doi-asserted-by":"publisher","DOI":"10.1002\/ange.201202952"},{"key":"e_1_2_6_13_3","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201202952"},{"key":"e_1_2_6_14_2","doi-asserted-by":"publisher","DOI":"10.1021\/nn2000367"},{"key":"e_1_2_6_15_2","doi-asserted-by":"publisher","DOI":"10.1002\/ange.201002994"},{"key":"e_1_2_6_15_3","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201002994"},{"key":"e_1_2_6_16_2","first-page":"3373","volume":"19","author":"Zhu B.","year":"2005","journal-title":"Synthesis"},{"key":"e_1_2_6_17_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja9707062"},{"key":"e_1_2_6_18_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja00344a056"},{"key":"e_1_2_6_19_2","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.77.3865"},{"key":"e_1_2_6_20_2","unstructured":"For the \u201cfulvalene effect\u201d see:"},{"key":"e_1_2_6_21_2","doi-asserted-by":"publisher","DOI":"10.1055\/s-2002-32572"},{"key":"e_1_2_6_22_2","doi-asserted-by":"publisher","DOI":"10.1021\/om00020a032"},{"key":"e_1_2_6_23_2","doi-asserted-by":"publisher","DOI":"10.1055\/s-1990-21140"},{"key":"e_1_2_6_24_2","doi-asserted-by":"publisher","DOI":"10.1021\/cr9003852"},{"key":"e_1_2_6_25_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.ccr.2009.02.013"},{"key":"e_1_2_6_26_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.ccr.2004.02.007"},{"key":"e_1_2_6_27_2","unstructured":"For the effect of polar groups on the strength of the metal\uf8ffcarbon bond see for example:"},{"key":"e_1_2_6_28_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja4080985"},{"key":"e_1_2_6_29_2","doi-asserted-by":"publisher","DOI":"10.1021\/om100974q"},{"key":"e_1_2_6_30_2","doi-asserted-by":"publisher","DOI":"10.1021\/jo9012223"},{"key":"e_1_2_6_31_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja901640m"},{"key":"e_1_2_6_32_2","doi-asserted-by":"publisher","DOI":"10.1021\/cr00102a004"},{"key":"e_1_2_6_33_2","unstructured":"There is tenuous (occasionally contradictory) evidence for M\uf8ffM bond weakening when replacing L=CO with L=donor often ascribed (L=PR3) to steric effects. See for example:"},{"key":"e_1_2_6_34_2","doi-asserted-by":"publisher","DOI":"10.1021\/om3003976"},{"key":"e_1_2_6_35_2","doi-asserted-by":"publisher","DOI":"10.1021\/om060768d"},{"key":"e_1_2_6_36_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.jorganchem.2005.06.015"},{"key":"e_1_2_6_37_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja974160v"},{"key":"e_1_2_6_38_2","doi-asserted-by":"publisher","DOI":"10.1080\/0095897021000036389"},{"key":"e_1_2_6_39_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja00249a017"},{"key":"e_1_2_6_40_2","doi-asserted-by":"publisher","DOI":"10.1021\/ic50186a070"},{"key":"e_1_2_6_41_2","doi-asserted-by":"publisher","DOI":"10.1039\/dt9770002352"},{"key":"e_1_2_6_42_2","doi-asserted-by":"publisher","DOI":"10.1039\/dt9770001302"},{"key":"e_1_2_6_43_2","doi-asserted-by":"publisher","DOI":"10.1039\/c39730000267"},{"key":"e_1_2_6_44_2","doi-asserted-by":"publisher","DOI":"10.1039\/JR9640001741"},{"key":"e_1_2_6_45_2","unstructured":"Taking 3 4\u2010di\u2010tert\u2010butylpyrrole as a model and a conservative estimate of its strain energy of 10.1\u2005kcal\u2009mol\u22121:"},{"key":"e_1_2_6_46_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0040-4020(01)82638-7"},{"key":"e_1_2_6_47_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0040-4039(00)97652-4"},{"key":"e_1_2_6_48_2","unstructured":"\u00a0"},{"key":"e_1_2_6_49_2","first-page":"696","volume-title":"Stereochemistry of Organic Compounds","author":"Eliel E. 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Vollhardt T.\u2005W. Weidman unpublished results."},{"key":"e_1_2_6_126_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.catcom.2004.03.005"},{"key":"e_1_2_6_127_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.molcata.2006.06.042"},{"key":"e_1_2_6_128_2","doi-asserted-by":"publisher","DOI":"10.1039\/ft9938901387"},{"key":"e_1_2_6_129_2","doi-asserted-by":"publisher","DOI":"10.1021\/ac60365a029"},{"key":"e_1_2_6_130_2","doi-asserted-by":"publisher","DOI":"10.1006\/jcis.1995.1367"},{"key":"e_1_2_6_131_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.molcata.2004.08.028"},{"key":"e_1_2_6_132_2","unstructured":"\u00a0"},{"key":"e_1_2_6_133_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.jhazmat.2012.04.039"},{"key":"e_1_2_6_134_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.molcata.2009.07.018"},{"key":"e_1_2_6_135_2","doi-asserted-by":"publisher","DOI":"10.1246\/bcsj.66.2385"},{"key":"e_1_2_6_136_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja01484a003"},{"key":"e_1_2_6_137_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja111411q"},{"key":"e_1_2_6_138_2","doi-asserted-by":"publisher","DOI":"10.1039\/c0sc00179a"},{"key":"e_1_2_6_139_2","doi-asserted-by":"publisher","DOI":"10.1021\/ic990794m"},{"key":"e_1_2_6_140_2","unstructured":"For selected reviews see:"},{"key":"e_1_2_6_141_2","doi-asserted-by":"publisher","DOI":"10.1590\/S0102-695X2007000200022"},{"key":"e_1_2_6_142_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0021-9673(00)85723-4"},{"key":"e_1_2_6_143_2","doi-asserted-by":"publisher","DOI":"10.1016\/0009-5907(66)80007-8"},{"key":"e_1_2_6_143_3","unstructured":"J.\u2005T. Dillon Y. Huang Abstracts of Papers 247th ACS National Meeting & Exposition Dallas TX USA March 16\u201320 2014 ANYL\u2010160."},{"key":"e_1_2_6_144_2","unstructured":"See for example:"},{"key":"e_1_2_6_145_2","doi-asserted-by":"publisher","DOI":"10.1039\/c3ta13092d"},{"key":"e_1_2_6_146_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.molstruc.2011.04.041"},{"key":"e_1_2_6_147_2","doi-asserted-by":"publisher","DOI":"10.1088\/0953-8984\/9\/34\/015"},{"key":"e_1_2_6_148_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0022-328X(02)01582-6"},{"key":"e_1_2_6_149_2","doi-asserted-by":"publisher","DOI":"10.1021\/cr940053x"},{"key":"e_1_2_6_150_2","unstructured":"SMART:Area\u2010Detector Software Package Bruker Analytical X\u2010ray Systems Inc. Madison WI 1995\u20131999."},{"key":"e_1_2_6_151_2","unstructured":"SAINT:SAX Area\u2010Detector Integration Program V. 7.06 Siemens Industrial Automation Inc. Madison WI 2005."},{"key":"e_1_2_6_152_2","unstructured":"XPREP: SHELXTL Crystal Structure Determination Package V. 6.12 Bruker AXS Inc. Madison WI 1995."},{"key":"e_1_2_6_153_2","unstructured":"SADABS: Siemens Area Detector ABSorption Correction Program V. 2.10 George Sheldrick 2005."},{"key":"e_1_2_6_154_2","unstructured":"XS: Program for the Solution of X\u2010ray Crystal Structures SHELXTL Crystal Structure Determination Package Bruker Analytical X\u2010ray Systems Inc. Madison WI 1995\u20131999."},{"key":"e_1_2_6_155_2","unstructured":"XL: Program for the Refinement of X\u2010ray Crystal Structures SHELXTL Crystal Structure Determination Package Bruker Analytical X\u2010ray Systems Inc. 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