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Herein, we demonstrate that sulfonated crown ether can form very stable host\u2010guest complexes with a series of push\u2010pull\u2010type photosensitizers, eventually leading to the dramatic fluorescence enhancement in visible and near\u2010infrared regions. Meanwhile, severe suppression in singlet oxygen (<jats:sup>1<\/jats:sup>O<jats:sub>2<\/jats:sub>) production is found, mainly due to the higher energy barriers between the excited single and triple states upon host\u2010guest complexation. Moreover, such complexation\u2010induced tuneable <jats:sup>1<\/jats:sup>O<jats:sub>2<\/jats:sub> generation systems has been utilized in adjusting the photochemical oxidation reactions of polycyclic aromatic hydrocarbons (anthracene) and sulfides ((methylthio)benzene) in water. This supramolecularly controlled photooxidation based on the selective molecular binding of crown ether with photosensitizers may provide a feasible and applicable strategy for monitoring and modulating many photocatalysis processes in aqueous phase.<\/jats:p>","DOI":"10.1002\/chem.202200005","type":"journal-article","created":{"date-parts":[[2022,2,7]],"date-time":"2022-02-07T05:55:30Z","timestamp":1644213330000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Induced Near\u2010Infrared Emission and Controlled Photooxidation based on Sulfonated Crown Ether in Water"],"prefix":"10.1002","volume":"28","author":[{"given":"Xiaoyun","family":"Dong","sequence":"first","affiliation":[{"name":"College of Chemistry State Key Laboratory of Elemento-Organic Chemistry Nankai University  Tianjin 300071 P. R. 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