{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,19]],"date-time":"2026-08-19T19:02:21Z","timestamp":1787166141450,"version":"build-2736575974"},"reference-count":187,"publisher":"Wiley","issue":"42","license":[{"start":{"date-parts":[[2022,6,8]],"date-time":"2022-06-08T00:00:00Z","timestamp":1654646400000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"content-domain":{"domain":["chemistry-europe.onlinelibrary.wiley.com"],"crossmark-restriction":true},"short-container-title":["Chemistry A European J"],"published-print":{"date-parts":[[2022,7,26]]},"abstract":"<jats:title>Abstract<\/jats:title>\n                  <jats:p>\n                    The reactivity of ferrocene\u2010based N\u2010heterocyclic tetrylenes [{Fe(\u03b7\n                    <jats:sup>5<\/jats:sup>\n                    \u2212C\n                    <jats:sub>5<\/jats:sub>\n                    H\n                    <jats:sub>4<\/jats:sub>\n                    \u2212NSi\n                    <jats:italic>t<\/jats:italic>\n                    BuMe\n                    <jats:sub>2<\/jats:sub>\n                    )\n                    <jats:sub>2<\/jats:sub>\n                    }E] (E=Ge, Sn, Pb) towards mesityl azide (MesN\n                    <jats:sub>3<\/jats:sub>\n                    ) is compared with that of PPh\n                    <jats:sub>2<\/jats:sub>\n                    \u2010functionalised congeners exhibiting two possible reaction sites, namely the E\n                    <jats:sup>II<\/jats:sup>\n                    and P\n                    <jats:sup>III<\/jats:sup>\n                    atom. For E=Ge and Sn the reaction occurs at the E\n                    <jats:sup>II<\/jats:sup>\n                    atom, leading to the formation of N\n                    <jats:sub>2<\/jats:sub>\n                    and an E\n                    <jats:sup>IV<\/jats:sup>\n                    =NMes unit. The germanimines are sufficiently stable for isolation. The stannanimines furnish follow\u2010up products, either by [2+3] cycloaddition with MesN\n                    <jats:sub>3<\/jats:sub>\n                    or, in the PPh\n                    <jats:sub>2<\/jats:sub>\n                    \u2010substituted case, by NMes transfer from the Sn\n                    <jats:sup>IV<\/jats:sup>\n                    to the P\n                    <jats:sup>III<\/jats:sup>\n                    atom. Whereas [{Fe(\u03b7\n                    <jats:sup>5<\/jats:sup>\n                    \u2212C\n                    <jats:sub>5<\/jats:sub>\n                    H\n                    <jats:sub>4<\/jats:sub>\n                    \u2212NSi\n                    <jats:italic>t<\/jats:italic>\n                    BuMe\n                    <jats:sub>2<\/jats:sub>\n                    )\n                    <jats:sub>2<\/jats:sub>\n                    }Pb] and other diaminoplumbylenes studied are inert even under forcing conditions, the PPh\n                    <jats:sub>2<\/jats:sub>\n                    \u2010substituted congener forms an addition product with MesN\n                    <jats:sub>3<\/jats:sub>\n                    , thus showing a behaviour similar to that of frustrated Lewis pairs. The germylenes of this study afford copper(I) complexes with CuCl, including the first structurally characterised linear dicoordinate halogenido complex [CuX(L)] with a heavier tetrylene ligand L.\n                  <\/jats:p>","DOI":"10.1002\/chem.202200996","type":"journal-article","created":{"date-parts":[[2022,5,5]],"date-time":"2022-05-05T05:36:21Z","timestamp":1651728981000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":20,"title":["Reactions of Mesityl Azide with Ferrocene\u2010Based N\u2010Heterocyclic Germylenes, Stannylenes and Plumbylenes, Including PPh\n                    <sub>2<\/sub>\n                    \u2010Functionalised Congeners"],"prefix":"10.1002","volume":"28","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-7694-1654","authenticated-orcid":false,"given":"Robin","family":"Guthardt","sequence":"first","affiliation":[{"name":"Institute of Chemistry University of Kassel  Heinrich-Plett-Stra\u00dfe 40 34132 Kassel Germany"},{"name":"Present address: School of Chemistry Monash University  PO Box 23 VIC 3800 Melbourne Australia"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lisa","family":"Oetzel","sequence":"additional","affiliation":[{"name":"Institute of Chemistry University of Kassel  Heinrich-Plett-Stra\u00dfe 40 34132 Kassel Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tobias","family":"Lang","sequence":"additional","affiliation":[{"name":"Institute of Chemistry University of Kassel  Heinrich-Plett-Stra\u00dfe 40 34132 Kassel Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Clemens","family":"Bruhn","sequence":"additional","affiliation":[{"name":"Institute of Chemistry University of Kassel  Heinrich-Plett-Stra\u00dfe 40 34132 Kassel Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8617-7768","authenticated-orcid":false,"given":"Ulrich","family":"Siemeling","sequence":"additional","affiliation":[{"name":"Institute of Chemistry University of Kassel  Heinrich-Plett-Stra\u00dfe 40 34132 Kassel Germany"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2022,6,8]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1002\/hlca.19190020164"},{"key":"e_1_2_8_2_1","unstructured":"Selected reviews:"},{"key":"e_1_2_8_3_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.chempr.2020.10.007"},{"key":"e_1_2_8_4_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.ccr.2008.08.009"},{"key":"e_1_2_8_5_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0040-4020(01)92229-X"},{"key":"e_1_2_8_6_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0040-4020(01)92417-2"},{"key":"e_1_2_8_7_1","unstructured":"\u00a0"},{"key":"e_1_2_8_8_2","doi-asserted-by":"publisher","DOI":"10.1002\/(SICI)1099-0682(199910)1999:10<1659::AID-EJIC1659>3.0.CO;2-I"},{"key":"e_1_2_8_9_2","doi-asserted-by":"publisher","DOI":"10.1021\/ja00996a027"},{"key":"e_1_2_8_10_1","first-page":"177","volume":"459","author":"\u00d6fele K.","year":"1993","journal-title":"Chem."},{"key":"e_1_2_8_11_1","unstructured":"Seminal paper:"},{"key":"e_1_2_8_12_2","doi-asserted-by":"publisher","DOI":"10.1039\/b508679e"},{"key":"e_1_2_8_13_2","doi-asserted-by":"publisher","DOI":"10.1039\/b401041h"},{"key":"e_1_2_8_14_1","unstructured":"\u00a0"},{"key":"e_1_2_8_15_2","doi-asserted-by":"publisher","DOI":"10.1002\/chem.201002805"},{"key":"e_1_2_8_16_2","doi-asserted-by":"publisher","DOI":"10.1002\/chem.200901203"},{"key":"e_1_2_8_17_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.200901046"},{"key":"e_1_2_8_17_3","doi-asserted-by":"publisher","DOI":"10.1002\/ange.200901046"},{"key":"e_1_2_8_18_2","doi-asserted-by":"publisher","DOI":"10.1021\/jo070789x"},{"key":"e_1_2_8_19_1","unstructured":"For reviews see:"},{"key":"e_1_2_8_20_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.196900201"},{"key":"e_1_2_8_20_3","doi-asserted-by":"publisher","DOI":"10.1002\/ange.19690810104"},{"key":"e_1_2_8_21_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.196706491"},{"key":"e_1_2_8_21_3","doi-asserted-by":"publisher","DOI":"10.1002\/ange.19670791504"},{"key":"e_1_2_8_22_1","unstructured":"For recent reviews see:"},{"key":"e_1_2_8_23_2","doi-asserted-by":"publisher","DOI":"10.1007\/s11172-021-3317-x"},{"key":"e_1_2_8_24_2","doi-asserted-by":"publisher","DOI":"10.1021\/jo100390p"},{"key":"e_1_2_8_25_1","unstructured":"\u00a0"},{"key":"e_1_2_8_26_2","first-page":"968","author":"Baldwin J. 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Steudel D. Scheschkewitz Chemistry of the Non-Metals: Syntheses\u2013Bonding\u2013Structures\u2013Applications De Gruyter Berlin Boston 2020 p. 139."},{"key":"e_1_2_8_94_1","doi-asserted-by":"publisher","DOI":"10.1039\/C39740000895"},{"key":"e_1_2_8_95_1","unstructured":"See for example:"},{"key":"e_1_2_8_96_2","doi-asserted-by":"publisher","DOI":"10.1039\/C8DT04295K"},{"key":"e_1_2_8_97_2","doi-asserted-by":"publisher","DOI":"10.1016\/S0022-328X(99)00010-8"},{"key":"e_1_2_8_98_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.199110172"},{"key":"e_1_2_8_98_3","doi-asserted-by":"publisher","DOI":"10.1002\/ange.19911030812"},{"key":"e_1_2_8_99_1","doi-asserted-by":"publisher","DOI":"10.1039\/c1dt11774b"},{"key":"e_1_2_8_100_1","first-page":"799","volume":"32","author":"Ding Y.","year":"2013","journal-title":"Chin. J. Struct. 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Chem."},{"key":"e_1_2_8_141_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201300461"},{"key":"e_1_2_8_141_3","doi-asserted-by":"publisher","DOI":"10.1002\/ange.201300461"},{"key":"e_1_2_8_142_1","unstructured":"Seminal paper:"},{"key":"e_1_2_8_143_2","doi-asserted-by":"publisher","DOI":"10.1515\/znb-1988-0103"},{"key":"e_1_2_8_144_2","doi-asserted-by":"publisher","DOI":"10.1039\/D0SC06364A"},{"key":"e_1_2_8_145_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.organomet.0c00348"},{"key":"e_1_2_8_146_2","doi-asserted-by":"publisher","DOI":"10.1039\/C4DT01794C"},{"key":"e_1_2_8_147_1","unstructured":"For CAAC complexes see:"},{"key":"e_1_2_8_148_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemmater.0c01769"},{"key":"e_1_2_8_149_2","doi-asserted-by":"publisher","DOI":"10.1039\/C6CC02349E"},{"key":"e_1_2_8_150_2","doi-asserted-by":"publisher","DOI":"10.1002\/chem.201500788"},{"key":"e_1_2_8_151_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.201500224"},{"key":"e_1_2_8_151_3","doi-asserted-by":"publisher","DOI":"10.1002\/ange.201500224"},{"key":"e_1_2_8_152_2","doi-asserted-by":"publisher","DOI":"10.1039\/C9RA04886C"},{"key":"e_1_2_8_153_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.jorganchem.2018.11.032"},{"key":"e_1_2_8_154_2","doi-asserted-by":"publisher","DOI":"10.1039\/c0dt00218f"},{"key":"e_1_2_8_155_2","doi-asserted-by":"publisher","DOI":"10.1021\/jo050397v"},{"key":"e_1_2_8_156_2","doi-asserted-by":"publisher","DOI":"10.1021\/om034285a"},{"key":"e_1_2_8_157_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.inorgchem.6b01505"},{"key":"e_1_2_8_158_1","doi-asserted-by":"publisher","DOI":"10.1002\/ejic.202000570"},{"key":"e_1_2_8_159_1","unstructured":"Selected reviews addressing redox-switchable ferrocene-based ligands:"},{"key":"e_1_2_8_160_2","doi-asserted-by":"publisher","DOI":"10.1039\/C9CC00795D"},{"key":"e_1_2_8_161_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.accounts.8b00523"},{"key":"e_1_2_8_162_2","doi-asserted-by":"publisher","DOI":"10.1039\/C5CS00096C"},{"key":"e_1_2_8_163_2","doi-asserted-by":"publisher","DOI":"10.1002\/zaac.200500270"},{"key":"e_1_2_8_164_2","doi-asserted-by":"publisher","DOI":"10.1002\/(SICI)1521-3773(19980420)37:7<894::AID-ANIE894>3.0.CO;2-L"},{"key":"e_1_2_8_164_3","doi-asserted-by":"publisher","DOI":"10.1002\/(SICI)1521-3757(19980403)110:7<936::AID-ANGE936>3.0.CO;2-X"},{"key":"e_1_2_8_165_1","doi-asserted-by":"publisher","DOI":"10.1021\/ic700457h"},{"key":"e_1_2_8_166_1","doi-asserted-by":"publisher","DOI":"10.1039\/dt9860001551"},{"key":"e_1_2_8_167_1","doi-asserted-by":"publisher","DOI":"10.1021\/om300909n"},{"key":"e_1_2_8_168_1","doi-asserted-by":"publisher","DOI":"10.1107\/S0108767307043930"}],"container-title":["Chemistry \u2013 A European Journal"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/chem.202200996","content-type":"application\/pdf","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/onlinelibrary.wiley.com\/doi\/full-xml\/10.1002\/chem.202200996","content-type":"application\/xml","content-version":"vor","intended-application":"text-mining"},{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/pdf\/10.1002\/chem.202200996","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2025,10,12]],"date-time":"2025-10-12T14:52:56Z","timestamp":1760280776000},"score":1,"resource":{"primary":{"URL":"https:\/\/chemistry-europe.onlinelibrary.wiley.com\/doi\/10.1002\/chem.202200996"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2022,6,8]]},"references-count":187,"journal-issue":{"issue":"42","published-print":{"date-parts":[[2022,7,26]]}},"alternative-id":["10.1002\/chem.202200996"],"URL":"https:\/\/doi.org\/10.1002\/chem.202200996","archive":["Portico"],"relation":{},"ISSN":["0947-6539","1521-3765"],"issn-type":[{"value":"0947-6539","type":"print"},{"value":"1521-3765","type":"electronic"}],"subject":[],"published":{"date-parts":[[2022,6,8]]},"assertion":[{"value":"2022-03-31","order":0,"name":"received","label":"Received","group":{"name":"publication_history","label":"Publication History"}},{"value":"2022-06-08","order":3,"name":"published","label":"Published","group":{"name":"publication_history","label":"Publication History"}}],"article-number":"e202200996"}}