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In this study, a new type of quasi\u2010solid polymer network electrolyte (SIPH\u2010x\u2010y%) was prepared by combining synthesized polymer network (SIPH) containing urethane bond linked ionic liquids (ILs), polyethylene glycol (PEG), and disulfide bond moieties, lithium bis(trifluoromethanesulfonyl)imide salt (LiTFSI), and glyme type additive. It was found that SIPH\u201020\u201040% was mechanically flexible, self\u2010healable, and showed high ionic conductivity of 2.67\u00d710<jats:sup>\u22124<\/jats:sup>\u2005S\u2009cm<jats:sup>\u22121<\/jats:sup>. Also, SIPH\u201020\u201040% possesses a high lithium ion transference number of 0.43 and good electrochemical stability. These properties enabled the SIPH\u201020\u201040% electrolyte membrane to support Li\/Li symmetrical cell to cycle stably during long term Li plating and stripping. The Li\/SIPH\u201020\u201040%\/LFP showed high delivered specific capacity and good stability (166.1\u2005mAh\u2009g<jats:sup>\u22121<\/jats:sup> after 106 cycles at 0.2\u2005C). Such glyme doped polymer network electrolyte provides new experimental findings for developing polymer\u2010based electrolyte with excellent mechanical integrity and battery related properties.<\/jats:p>","DOI":"10.1002\/chem.202202717","type":"journal-article","created":{"date-parts":[[2022,9,23]],"date-time":"2022-09-23T08:10:35Z","timestamp":1663920635000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":6,"title":["Self\u2010Repairable and Flexible Polymer Network Electrolyte with Enhanced Lithium\u2010Ion Conduction for Lithium Metal Batteries"],"prefix":"10.1002","volume":"28","author":[{"given":"Yaduo","family":"Song","sequence":"first","affiliation":[{"name":"School of Electronic Science and Engineering University of Electronic Science and Technology of China  Chengdu 611731 P. R. 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