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In order to augment the Lewis acidity of these newly formed unsymmetrical monotellurides, these have been transformed into corresponding unsymmetrical 2\u2010\n                    <jats:italic>N<\/jats:italic>\n                    \u2010(quinolin\u20108\u2010yl)benzamide tellurium cations. Subsequently, these Lewis acidic tellurium cations were used as chalcogen bonding catalysts, enabling the synthesis of various substituted 1,2\u2010dihydroquinolines by activating ketones with anilines under mild conditions. Moreover, the synthesized 2\u2010\n                    <jats:italic>N<\/jats:italic>\n                    \u2010(quinolin\u20108\u2010yl)benzamide phenyl tellurium cation has also catalyzed the formation of\n                    <jats:italic>\u03b2<\/jats:italic>\n                    \u2010amino alcohols in high regioselectivity by effectively activating epoxides at room temperature. Mechanistic insight by\n                    <jats:sup>1<\/jats:sup>\n                    H and\n                    <jats:sup>19<\/jats:sup>\n                    F NMR study, electrostatic surface potential (ESP map), control reaction in which tellurium cation reacted explosively with epoxide, suggested that the enhanced Lewis acidity of tellurium center seems responsible for efficient catalytic activities under mild conditions enabling\n                    <jats:italic>\u03b2<\/jats:italic>\n                    \u2010amino alcohols with excellent regioselectivity and 1,2\u2010dihydroquinolines with trifluoromethyl\n                    <jats:sub>,<\/jats:sub>\n                    nitro, and pyridylsubstitution, which were difficult to access.\n                  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