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However, inherent drawbacks of soybean meal adhesives, such as poor toughness, low bond strength, and susceptibility to mold, have hindered their further development. In this study, a novel biomass adhesive, SM\u2010MMT@TA, was developed based on supramolecular interactions between tannic acid (TA), montmorillonite (MMT), and soybean meal. Tannic acid was securely attached to the MMT surface through coordination bonds with Ca\n                    <jats:sup>2+<\/jats:sup>\n                    , Mg\n                    <jats:sup>2+<\/jats:sup>\n                    , and Al\n                    <jats:sup>3+<\/jats:sup>\n                    ions, enhancing MMT's compatibility in the matrix via strong interfacial interactions. TA on the surface of MMT@TA effectively bonded with soy protein through strong hydrogen bonding, thereby increasing the crosslink density. As a result, the adhesive exhibited a wet shear strength of up to 1.75\u2005MPa, which represents a 143.05\u2009% increase compared to unmodified SM adhesive. Moreover, the moisture absorption rate of the adhesive was reduced to 26.79\u2009%. Furthermore, abundant non\u2010covalent interactions improved the adhesive's toughness, while natural polyphenols provided additional mold resistance. Overall, this study presents a new strategy for developing renewable, high\u2010performance biomass\u2010based adhesives.\n                  <\/jats:p>","DOI":"10.1002\/chem.202402718","type":"journal-article","created":{"date-parts":[[2024,12,5]],"date-time":"2024-12-05T04:45:26Z","timestamp":1733373926000},"update-policy":"https:\/\/doi.org\/10.1002\/crossmark_policy","source":"Crossref","is-referenced-by-count":5,"title":["Soy Protein Adhesive Enhanced Through Supramolecular Interaction with Tannic Acid Modified Montmorillonite"],"prefix":"10.1002","volume":"31","author":[{"given":"Yanyan","family":"Bian","sequence":"first","affiliation":[{"name":"State Key Laboratory of Efficient Production of Forest Resources MOE Key Laboratory of Wood Material Science and Application &amp; Beijing Key Laboratory of Wood Science and Engineering Beijing Forestry University  Beijing 100083 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Qinghua","family":"Guo","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Efficient Production of Forest Resources MOE Key Laboratory of Wood Material Science and Application &amp; Beijing Key Laboratory of Wood Science and Engineering Beijing Forestry University  Beijing 100083 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jinfeng","family":"Cao","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Efficient Production of Forest Resources MOE Key Laboratory of Wood Material Science and Application &amp; Beijing Key Laboratory of Wood Science and Engineering Beijing Forestry University  Beijing 100083 China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4590-2919","authenticated-orcid":false,"given":"Jianzhang","family":"Li","sequence":"additional","affiliation":[{"name":"State Key Laboratory of Efficient Production of Forest Resources MOE Key Laboratory of Wood Material Science and Application &amp; Beijing Key Laboratory of Wood Science and Engineering Beijing Forestry University  Beijing 100083 China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"311","published-online":{"date-parts":[[2024,12,10]]},"reference":[{"key":"e_1_2_8_1_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-023-06507-5"},{"key":"e_1_2_8_2_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jclepro.2024.141474"},{"key":"e_1_2_8_3_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesb.2023.111169"},{"key":"e_1_2_8_4_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2023.121093"},{"key":"e_1_2_8_5_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.jclepro.2022.132460"},{"key":"e_1_2_8_6_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesb.2022.109744"},{"key":"e_1_2_8_7_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijbiomac.2024.129520"},{"key":"e_1_2_8_8_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.indcrop.2022.114982"},{"key":"e_1_2_8_9_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.mtcomm.2023.106426"},{"key":"e_1_2_8_10_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.polymertesting.2020.106648"},{"key":"e_1_2_8_11_1","doi-asserted-by":"publisher","DOI":"10.3390\/molecules23112752"},{"key":"e_1_2_8_12_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijbiomac.2023.127669"},{"key":"e_1_2_8_13_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijbiomac.2022.08.028"},{"key":"e_1_2_8_14_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2022.135442"},{"key":"e_1_2_8_15_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.ijadhadh.2023.103442"},{"key":"e_1_2_8_16_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.compositesb.2022.110049"},{"key":"e_1_2_8_17_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cej.2022.135437"},{"key":"e_1_2_8_18_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2014.08.106"},{"key":"e_1_2_8_19_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.polymertesting.2023.108221"},{"key":"e_1_2_8_20_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-24835-w"},{"key":"e_1_2_8_21_1","doi-asserted-by":"publisher","DOI":"10.1002\/adfm.202405016"},{"key":"e_1_2_8_22_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.carbpol.2019.05.090"},{"key":"e_1_2_8_23_1","doi-asserted-by":"publisher","DOI":"10.1016\/j.tifs.2023.104148"},{"key":"e_1_2_8_24_1","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.1c00815"},{"key":"e_1_2_8_25_1","doi-asserted-by":"publisher","DOI":"10.1038\/s41586-023-06335-7"},{"key":"e_1_2_8_26_1","author":"Zeng G.","year":"2022","journal-title":"Chem. 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